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Identifying quantum resources in encoded computations
That author's affiliation: École Normale Supérieure - PSL Institution (first & last author): École Normale Supérieure - PSL
Identifying quantum resources in encoded computations
Gold keeps glittering courtesy of surface chemistry
Hexagonal patterns on the surface of gold crystals are an unfavourable environment for reactions.
MATBG Josephson diode as an universal thermal machine
Magic-angle twisted bilayer graphene Josephson junctions (MATBG-JJ) with a gate-tunable valley-polarized weak link exhibit an intrinsic Josephson diode effect originating from broken symmetries associated with valley polarization and band-structure anisotropy. Exploiting this nonreciprocal superconducting platform, we construct quantum Stirling (QSC), Otto (QOC), and Carnot (QCC) thermodynamic cycles, where the valley-polarization potential $\Delta_v$ acts as the principal control parameter, in contrast to conventional Josephson thermal machines driven by superconducting phase bias. We systematically compare the performance of MATBG-based Josephson diode thermal machines (MATBG-JDTM) with MATBG-based Josephson junction thermal machines (MATBG-JJTM) and AA-stacked bilayer graphene Josephson junction thermal machines (AABLG-JJTM). Owing to the flat-band-enhanced density of states and electrically tunable nonreciprocal transport in MATBG, both MATBG-JDTM and MATBG-JJTM exhibit significantly enhanced work output and efficiency over a broad operating regime compared to AABLG-JJTM. In particular, the gate-controlled MATBG-JDTM provides a flux-free alternative to conventional phase-driven architectures, mitigating limitations associated with magnetic-flux control and flux-noise effects. Our results establish MATBG Josephson diode platforms as a promising route toward electrically tunable quantum thermal machines and nonreciprocal superconducting caloritronics.
Spin-Hall-Like Magnon Transport in a Synthetic Antiferromagnetic Skyrmion Lattice
We investigate spin-Hall-like magnon edge transport in a synthetic antiferromagnetic skyrmion lattice composed of two antiferromagnetically coupled skyrmion lattice layers with opposite magnetic textures. Based on a relaxed bilayer texture from micromagnetic simulations, we construct the bosonic Bogoliubov-de Gennes Hamiltonian within linear spin-wave theory and calculate the bulk and strip magnon spectrum. We find counterpropagating in-gap edge modes with opposite layer polarization, whose layer-resolved propagation is further confirmed by dynamical micromagnetic simulations. A symmetry analysis shows that the fully coupled system lacks the pseudo-time-reversal symmetry required for a genuine bosonic Z2 topological phase. Thus, the observed edge modes are not Z2-protected helical magnon edge states, but layer-polarized, spin-Hall-like modes originating from the opposite Hall tendencies of the two skyrmion lattice layers. These results establish synthetic antiferromagnetic skyrmion lattices as a platform for spin-Hall-like magnon transport beyond a strict bosonic Z2 classification.
Quantum anomalous Hall effect in chiral semimetals
The quantum anomalous Hall (QAH) effect is conventionally understood to exist only in Chern insulators, while a recent study has shown that ferromagnetic metals can also host the QAH effect. Between insulators and metals, we demonstrate that QAH can persist even in a chiral semimetal, where conduction and valence bands touch at zero energy. Transport calculations demonstrate that the Hall conductivity of such a system can be quantized in the presence of dephasing. Interestingly, its longitudinal conductivity remains finite and exhibits semimetallic behavior, in contrast to Chern insulators. This unusual transport behavior originates from the quantization of the Berry curvature integral over occupied states and the semimetallic band structure. This chiral semimetal can transition into a Chern insulator, accompanied by the vanishing of longitudinal conductivity and a reduction of the intrinsic length scale of the Hall response. Our results extend the concept of QAH and uncover the semimetallic QAH transport signatures.
Photon correlation microscopy of quantum matter
Light and matter share fundamental statistical properties, yet the experimental probes of quantum optics and many-body physics have largely evolved along separate trajectories. While many-body physics explores emergent collective phenomena, quantum optics has refined the measurement of correlations between individual photons. Here, we introduce photon correlation microscopy (PCM) - which bridges the two domains by leveraging correlations of emitted light to probe the correlations in quantum matter at mesoscopic scales. We demonstrate this approach using a one-dimensional (1D) ensemble of dipolar excitons confined at a lateral monolayer MoSe$_2$-WSe$_2$ heterojunction. We use gate-defined potentials to confine the 1D excitons to a mesoscopic lengthscale to enhance the visibility of matter correlations in the emitted photon field. Power-dependent spectroscopy reveals a transition from a compressible to an incompressible phase, signaled by the simultaneous saturation of the emission intensity and energy blueshift, which is supported by numerical simulations. Through this crossover, photon correlation measurements show a striking evolution from bunching at low densities to antibunching at high densities. This constitutes a many-body blockade of photon emission emerging directly from a number-stabilized state, driven by collective dipolar repulsion. Our results establish PCM as a powerful probe of many-body physics through the lens of quantum optics, extensible to a broad class of correlated electronic phases, while pointing toward a route to generating non-classical light through many-body correlations.
Zero modes of non-abelian Dirac operator in topologically non-trivial band insulator
We show that the local gauge-invariance of the quantum geometric tensor (QGT) defined in the Block-momentum space of a generic $N$-level (sublattice degrees of freedom) band insulator implies the existence of zero modes of non-abelian Dirac operator in such momentum space. Solutions of these zero modes equations in the two-dimensional Brillouin zone torus, in terms of Jacobi Theta function determine the probability amplitudes associated with the $N$-component ground state wave-function under adiabatic approximation in this Hilbert space. These solutions subjected to normalization, defines a complex projective ($CP$) space of $N-1$ dimension ($CP^{N-1}$ space) when one or more degeneracy points exist in the dispersion spectrum of such band-isulator. We show how the non-abelian generalization of the vortexability criterion of Chern bands automatically follows from these zero-mode equations, and also demonstrate their connection with momentum space-version of Lowest landau level algebra. Subsequently we write an Euclidean action from which these zero mode equations follow. We point out that the non-interacting part of different paradigms used to understand fractional Chern insulator(FCI) like phases in a host of two-dimensional material can be understood within this approach. We analyse two effective hamiltonian : lattice Dirac (QZW) model and two-band model for rhombohedral $N$-layer graphene in our propsoed framework and obtain important conclusions.
Full Quantum and Mixed Quantum--Classical Dynamics of Hot Exciton Cooling in Semiconductor Nanocrystals
Hot-exciton relaxation in semiconductor nanocrystals (NCs) is often described using perturbative theories, but their accuracy is difficult to assess for realistic exciton--phonon Hamiltonians. Here, we benchmark the perturbative quantum master equation (QME) and several mixed quantum--classical (MQC) methods against fully quantum mechanical dynamics. Using atomistically parameterized models for CdSe core and CdSe/CdS core--shell NCs, we find that bare CdSe exhibits an ultrafast initial decay followed by slower cooling, whereas the core--shell system is dominated by the slower component. Analysis of reduced models shows that the ultrafast component arises from rapid diabatic state mixing driven by thermal fluctuations of low-frequency phonons, rather than from nuclear-assisted energy relaxation. The QME captures the initial fast decay but can fail for the slower relaxation in the diabatic representation, while the mapping approach to surface hopping (MASH) gives the most consistent agreement with both benchmark dynamics and equilibrium populations. These results establish a benchmark for exciton-cooling dynamics in NCs and clarify the physical regimes in which widely used approximate methods are reliable.
Deterministic Electrical Switching in Altermagnets via Surface Antisymmetry Groups
A surface antisymmetry group framework is developed to establish design rules for deterministic electrical switching of the N\'eel vector in a film of a collinear bipartite antiferromagnet. In centrosymmetric altermagnets, where current-induced spin-orbit torques vanish in the bulk, staggered effective fields can nevertheless exist as a macroscopic interfacial response, whose allowed tensor form is determined by the surface antisymmetry point group for the given surface orientation. Separately, the structure of the spin conductivity tensor determines which surface orientations allow transverse spin current generation via the nonrelativistic spin-splitter effect. Taken together, these symmetry-enforced properties establish which surface orientations of $d$-wave altermagnets can serve as deterministically switchable spin current sources in spin-torque heterostructures. Because the design rules are based solely on the surface antisymmetry point group, the symmetry-allowed staggered effective fields are robust against averaging over equilibrium surface roughness.
Quantum criticality of the ferromagnetic Dicke-Ising model
We describe the quantum phase transitions in the ferromagnetic Dicke-Ising model using a Landau theory approach. The theory quantitatively captures the change from a second- to a first-order transition between the normal and superradiant phases through a tricritical point. We identify virtual correlated nearest-neighbor double spin-flip processes as the crucial mechanism responsible for this behavior. The tricritical point constitutes a quantum phase transition above the upper critical dimension. We discuss the modifications to finite-size scaling required for the correct interpretation of numerical data at the tricritical point. Our results emphasize the need for adapted finite-size scaling forms in all-to-all interacting quantum systems and establish the ferromagnetic Dicke-Ising model as a paradigmatic platform for quantum phase transitions above the upper critical dimension, encompassing both standard $\phi^4$ criticality and beyond.
Inelastic Neutron Scattering of the layered Kitaev ferromagnet Li$_3$Co$_2$SbO$_6$
Cobalt-based quantum magnets forming layered honeycomb arrangements have attracted much attention recently, as they are considered as a potential platform for materials with exotic Kitaev spin exchange. Amongst the discussed candidate materials are Na$_3$Co$_2$SbO$_6$ and Na$_2$Co$_2$TeO$_6$, both possessing a low-temperature ground state with magnetic zigzag ordering, similar to Na$_2$IrO$_3$ and $\alpha$-RuCl$_3$. Here we report inelastic neutron scattering experiments on the quantum magnet Li$_3$Co$_2$SbO$_6$, which features ferromagnetic honeycomb planes with opposite magnetizations in neighboring planes. By comparing with linear spin wave theory, we show that the magnetic properties of Li$_3$Co$_2$SbO$_6$ can be well-modelled by an extended Kitaev--Heisenberg model, establishing it as a Kitaev-ferromagnet, or more specifically, as a Kitaev A-type antiferromagnet. Our analysis is complemented by magnetic field measurements and simulations.
Direction-selective intertwined charge, orbital, and lattice orders under uniaxial strain in hole-doped manganite: La0.75Ca0.25MnO3
The complex interplay of charge, spin, orbital, and lattice degrees of freedom governs emergent phases in quantum materials, making strain a powerful control parameter. Recent advances in free-standing layer techniques have enabled extreme strains of nearly 8%, opening access to novel and often unexpected electronic and magnetic phases. Here, using a density functional theory approach, we investigate the effect of direction-selective uniaxial strain on the prototypical Jahn-Teller system La1-xCaxMnO3 (x = 0.25). We find that different strain directions stabilize qualitatively distinct structural, charge, and orbital responses, rather than merely different strengths of the same phase. In particular, extreme uniaxial strain selectively induces cooperative Jahn-Teller, breathing-like, and site-selective modulations, thereby enabling previously inaccessible intertwined orders in manganites. These results establish direction-selective uniaxial strain as a powerful and selective route for engineering emergent phases in quantum materials.
Cascade of magnetic-field-induced quantum spin states in a spin-1 honeycomb magnet
That author's affiliation: University of Science and Technology of China Institution (first & last author): University of Science and Technology of China
Quantum fluctuations endow spin systems with surprisingly enriched magnetic phase diagrams. In frustrated magnets, strong quantum fluctuations boosted by either geometrical incompatibility or competitive exchange interactions stabilize cascades of unusual phases of matter. Here we reveal the presence of multiple quantum phases in the honeycomb antiferromagnet Na$_{3}$Ni$_{2}$BiO$_{6}$, both inside and beyond its field-induced one-third magnetization plateau. Comprehensive measurements of thermodynamic quantities demonstrate that the one-third plateau comprises at least three distinct spin states with nearly-degenerate net magnetization, separated by first-order transitions that likely involve sequential spin reconfiguration. Upon further increasing the magnetic field, the system evolves across a myriad of peculiar phases before reaching full polarization; these intermediate phases possess copious low-energy excitations, manifested by anomalous upturns of specific heat at ultralow temperatures -- probably hinting at the development of "hidden" ordered ground states. The complex magnetic phase diagram of Na$_{3}$Ni$_{2}$BiO$_{6}$ underlines the preponderant impact of quantum fluctuations on a honeycomb spin lattice with strong exchange frustration.
Topological lattice gauge theory enriched by non-invertible symmetry
We use finite group topological lattice gauge theory, also known as the quantum double model, as a lens to explore a notion of topological order enriched by a non-invertible symmetry. For invertible symmetry enriched topological order, there is an established axiomatisation in terms of a G-crossed braided fusion category. We lay the foundations for a generalisation of this notion. By condensing an arbitrary algebra of charges in a quantum double model, we demonstrate that the category of localised excitations in the resulting theory forms a hypergroup-graded extension of the category of deconfined excitations. For every element in the hypergroup, the associated domain wall acts in a typically non-invertible way on these localised excitations. Both this action and the monoidal structure are compatible with the hypergroup grading. The actual categorical action is encoded in a Hopf monad on the category of localised excitations, and gauging the non-invertible symmetry amounts to computing the category of modules over this Hopf monad. Finally, we outline how this framework naturally extends to theories obtained by condensing algebras in a generic string-net model.
Odd spin symmetry and anisotropy switching in p-wave magnet CeNiAsO
Odd-parity magnets, complementary to altermagnets, exhibit unique properties such as high efficiency in charge-spin conversion and compatibility with conventional superconductivity, of critical importance in the pursuit of energy-efficient spintronics and topological superconductors for quantum computation. For even-parity d-wave and g-wave altermagnets, the magnetic structure, spin-split band structure and physical properties are currently under intensive study. On the contrary, while hundreds of odd-parity magnets and the promising properties have been predicted in theory, experimental studies are scarce. Specifically, the magnetic structure and transport properties of candidates NiI2 and Ga3Ru4Al12 have been reported, yet the characteristic band structure and particularly the odd-parity spin symmetry remain elusive. Here we demonstrate experimentally the deterministic p-wave spin symmetry and resistance anisotropy switching for the prototype odd-parity magnet, CeNiAsO. Angle-resolved photoemission spectroscopy (ARPES) reveals two cleaved terminations with distinct surface band structure. By compensating the polar surface, we achieve intrinsic bulk band structure, for which the spin splitting can be well described by the p-wave magnetic structure through first-principles calculation. The bulk spin polarization measured by spin-resolved ARPES exhibits symmetry with only one degenerate plane, fingerprint of p-wave magnetism. We further demonstrate giant resistance anisotropy and switching between high-resistance and low-resistance states through modest field-induced domain selection, highlighting its potential for antiferromagnetic spin memory devices. The structural similarity between CeNiAsO and 1111-type Fe-based superconductors stimulates further exploration on the interplay between p-wave magnetism, superconductivity and band topology.
Thermodynamic-limit dispersion relations on trapped-ion quantum hardware
We run a numerical linked-cluster expansion with a quantum algorithm (NLCE+QA), computing ground-state energies and one quasi-particle dispersions in the thermodynamic limit using a 20-qubit trapped-ion quantum processing unit (QPU). The NLCE+QA framework extracts thermodynamic-limit properties from small-cluster calculations, making it naturally suited for near-term quantum devices. Projector-based block-diagonalization schemes such as projective cluster-additive transformation (PCAT) are essential to NLCE+QA, and they involve matrix inversion and square root operations that amplify measurement noise. A central question is therefore whether current hardware can provide expectation values that are accurate enough to withstand non-linear classical post-processing. We explore this challenge for the transverse-field Ising model (TFIM) in one dimension, on a ladder geometry, as well as in a longitudinal field in one dimension. For the quantum algorithm, we consider adiabatic state preparation (ASP), as well as a variational quantum eigensolver (VQE) trained on a classical device. The final expectation values are obtained from the QPU, using a novel alternative to the Hadamard test that we name the CX-test. We explore the regimes currently attainable on quantum devices and comment on the improvements needed for quantum computers to achieve results beyond classical reach.
Disorder-induced proximate quantum spin ice phase in Pr2Sn2O7
Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood. Here we combine bulk characterization and single-crystal neutron-scattering measurements to investigate the non-Kramers pyrochlore Pr2Sn2O7. At temperatures below ~1 K, the system exhibits key hallmarks of quantum spin-ice physics, including anisotropic spin-ice correlations and two distinct dynamical timescales. Upon further cooling, however, we observe a complete spin-freezing transition at T_f ~ 0.15 K, accompanied by recovery of the full nuclear Schottky anomaly, the emergence of a gapped magnetic excitation, and the development of incipient (100) magnetic correlations. Comparison with related Pr-based pyrochlores places Pr2Sn2O7 near the spin-frozen boundary of a disorder-perturbed phase diagram. These results establish a disorder-driven framework for how quantum spin-ice behavior evolves into frozen ground states, demonstrating that proximity to a quantum spin liquid can coexist with disorder-induced spin freezing in non-Kramers pyrochlores.
Quantum Cellular Automata on Symmetric Subalgebras
We investigate quantum cellular automata (QCA) on one-dimensional spin systems defined over a subalgebra of the full local operator algebra - the symmetric subalgebra under a finite Abelian group symmetry $G$. For systems where each site carries a regular representation of $G$, we establish a complete classification of such subalgebra QCAs based on two topological invariants: (1) a surjective homomorphism from the group of subalgebra QCAs to the group of anyon permutation symmetries in a $(2+1)d$ $G$ gauge theory; and (2) a generalization of the Gross-Nesme-Vogts-Werner (GNVW) index that characterizes the flow of the symmetric subalgebra. Specifically, two subalgebra QCAs correspond to the same anyon permutation and share the same index if and only if they differ by a finite-depth unitary circuit composed of $G$-symmetric local gates. We also identify a set of operations that generate all subalgebra QCAs through finite compositions. As an example, we examine the Kramers-Wannier duality on a $\mathbb{Z}_2$ symmetric subalgebra, demonstrating that it maps to the $e$-$m$ permutation in the two-dimensional toric code and has an irrational index of $\sqrt{2}$. Therefore, it cannot be extended to a QCA over the full local operator algebra and mixes nontrivially with lattice translations.
Atomic-Scale Observation of Symmetry Breaking in Altermagnetic MnTe
The recent discovery of altermagnetism has sparked growing interest in compensated magnetic systems as promising platforms for highly scalable spintronics. Altermagnetism is a distinct magnetic order where opposite spin sublattices are connected by rotation, yielding zero net magnetization but momentum-dependent spin splitting. To date, experimental verification of altermagnetic order has been achieved predominantly through bulk-sensitive techniques, including spin-dependent electronic spectra and transport responses. However, direct atomic-scale evidence that explicitly correlates crystal symmetry, local structural distortions, and magnetic ordering has remained unexplored. Here, we report the direct atomic-scale observation of coexisting polar distortions and altermagnetic order in MnTe, combining atomic resolution scanning transmission electron microscopy (STEM) imaging with electron magnetic chiral dichroism (EMCD) measurements. We reveal that MnTe is not an ideal uniform P63/mmc g-wave altermagnet at the atomic scale. Instead, it hosts ubiquitous inversion-symmetry-breaking distortions that lower the spin-space-group (SSG) symmetry, admits d-wave altermagnetic components, and in lower-symmetry regimes, even allow s-wave spin splitting (net magnetization). The coexistence of ferroelectric signatures and altermagnetic order establishes local lattice symmetry in MnTe as a control knob for altermagnetic spin splitting, spin current generation, and multiferroic memory applications.
Quantum Printing: Laguerre-Gaussian Beam Induced Topological Magnetic Textures
Structured light has become a practical tool for controlling matter by applying tailored, space- and time-dependent electromagnetic fields. We show that Laguerre-Gaussian pulses imprint non-collinear magnetic textures via the spatial structure of optical magnetic field. Our route offers a direct spatial selectivity determined by the optical features without relying on material anisotropic interactions. The proposed printing approach does not require interfacial anisotropy or bulk chirality, current-driven torques, or thermal quenching. We use micromagnetic simulations to demonstrate the potential to create topological charge density emerging during the pulse and reveal control through the optical topological properties and polarization. These results suggest structured-light quantum printing as a viable approach for magnonics and motivate studies toward reconfigurable topological textures enabled by ultrafast THz optics and non-thermal control.
Tuning quantum tunneling in WSe$_2$ via strain engineering
We present a comprehensive theoretical study of strain-engineered quantum transport in monolayer tungsten diselenide (WSe$_2$) in the presence of an electrostatic scalar potential. By incorporating strain effects within a low-energy Dirac framework, we analyze their impact on spin- and valley-resolved transmission, conductance, and polarization. The applied potential barrier partitions the system into three distinct regions, allowing for an analytical derivation of the wave functions in each domain. Enforcing continuity conditions at the interfaces yields exact expressions for the transmission and reflection amplitudes. The transmission probability is evaluated from the corresponding current densities, while the conductance is obtained using the Landauer-B\"uttiker formalism, enabling a quantitative determination of spin and valley polarizations. Our numerical analysis reveals that strain acts as a powerful tuning parameter that reshapes the electronic dispersion and strongly modifies transport characteristics. In particular, the transmission and conductance exhibit pronounced oscillatory behavior driven by quantum interference and resonant tunneling mechanisms. More importantly, both spin and valley polarizations display substantial and highly controllable variations as functions of strain, barrier height, and incident energy. These results demonstrate that strain and electrostatic engineering provide an efficient and versatile platform for manipulating spin-valley degrees of freedom in WSe$_2$. The ability to tailor polarization and interference effects suggests promising opportunities for the design of next-generation spintronic, valleytronic, and optoelectronic devices based on two-dimensional transition-metal dichalcogenides.
Non-magnetic spin splitting driven by spin-valley-layer coupling in multilayer WSe2
Transition metal dichalcogenides provide a platform for exploring spin-valley physics, offering a promising approach to electric-field-driven spin control for low-power spintronic and quantum devices. Here, we demonstrate electric-field-induced spin splitting in the Q and Q' valleys of multilayer n-type WSe2 using quantum-point-contact spectroscopy. Systematic modulations in four distinct conductance quantization steps, providing direct evidence of spin-valley-layer coupling-driven spin-resolved density of states, are achieved by tuning the out-of-plane gate voltage. Notably, the electric-field-induced spin splitting significantly dominate the magnetic-field-induced valley-Zeeman effect (i.e., ~7 meV for a displacement field change of ~0.08 V/nm vs. ~2 meV for a magnetic field of B = 9 T), demonstrating a powerful, non-magnetic manipulation of spin states. This ability to manipulate spin states by gate voltage is crucial for advancing next-generation low-power spintronic and quantum information technologies.
Time reversal reserved spin valve and spin transistor based on unconventional $p$-wave magnets
The anisotropic spin splitting in unconventional magnets opens new opportunities for realizing spintronic functionalities without relying on net magnetization or relativistic spin-orbit coupling. Here, we propose a spin valve and a spin transistor based on unconventional $p$-wave magnets (UPMs). The spin valve is realized in a junction where a normal metal is sandwiched between two UPMs whose exchange-field strength vectors are oriented transverse to the junction direction. The conductance of such a device is governed by the spin alignment between two UPMs: when their strength vectors are parallel, the spin-state alignment enables efficient electron transmission, leading to a high-conductance state; in contrast, the antiparallel configuration suppresses the conductance owing to the opposite spin orientations. Furthermore, the spin-valve can be extended to a spin transistor by replacing the central normal metal with another UPM with a longitudinally oriented strength vector and a perpendicular spin polarization axis. The central UPM enables uniform spin precession with the same precession frequency for all transverse modes. Both devices can be electrically controlled by modulating the strength vectors of UPMs. These findings establish UPMs as a promising platform for developing spintronic devices without net magnetization or relativistic spin-orbit coupling.
Breakdown of Topological Inheritance and Twist-Induced Quantum Geometry Reconfiguration in Moir\'e Flat Bands
Since the inception of moir\'e quantum matter, a foundational tenet of the field has been that the quantum geometry of emergent flat bands is faithfully inherited from the low-energy valleys of the constituent monolayers. Here, we demonstrate a breakdown of this longstanding tenet in twisted bilayers of loop-current-ordered kagome lattices (tb-LCK). Using microscopic tight-binding modeling, we reveal a twist-induced reconfiguration of quantum geometry where realistic interlayer hybridization quenches topological inheritance from the monolayer. By tuning the loop-current phase, we identify distinct regimes in which the monolayer Berry curvature is either substantially redistributed or entirely suppressed in the moir\'e flat bands. We further show that this quantum geometric collapse is expected to be readily accessible in vanadium-based kagome metals such as AV$_{\text{3}}$Sb$_{\text{5}}$, and that Floquet engineering via waveguide laser illumination offers a practical route to turn topological inheritance on and off. Our findings uncover a universal mechanism for quantum geometric reconstruction, establishing interlayer coupling strength as an independent parameter for tuning band topology beyond the weakly coupled van der Waals heterostructure paradigm.
Quantum jumps in open cavity optomechanics and Liouvillian versus Hamiltonian exceptional points
Exceptional points, where two or more eigenstates of a non-Hermitian system coalesce, are now of interest across many fields of physics, from the perspective of open-system dynamics, sensing, nonreciprocal transport, and topological phase transitions. In this work, we investigate exceptional points in cavity optomechanics, a platform of interest to diverse communities working on gravitational-wave detection, macroscopic quantum mechanics, quantum transduction, etc. Specifically, we clarify the role of quantum jumps in making a clear distinction between Liouvillian and Hamiltonian exceptional points in optomechanical systems. While the Liouvillian exceptional point arises from the unconditional Lindblad dynamics and is independent of the phonon-bath temperature, the Hamiltonian exceptional point emerges from the conditional no-jump evolution and acquires a thermal shift due to an enhanced conditional damping. Employing the thermofield formalism, we derive a unified spectral framework that interpolates between these regimes via an analytical hybrid-Liouvillian description. Remarkably, in the weak-quantum-jump regime, the exceptional point is perturbed only at the second order, highlighting the robustness of the Hamiltonian exceptional point under small hybrid perturbations. Our work reveals a continuous family of hybrid exceptional points, clarifies the operational and physical differences between the conditional and unconditional dissipative dynamics in optomechanical systems, and provides a probe for thermal baths.
Robust spin-squeezing with random interaction graphs: the lesson from universality
We establish the conditions under which scalable spin squeezing can be achieved in interacting spin ensembles embedded in arbitrary, inhomogeneous graph geometries. We identify two different forms of squeezing: OAT-like scalable squeezing is governed solely by the universal properties of the interaction graph and is controlled by its spectral dimension. In critical squeezing, on the other hand, the value of the spectral dimension only furnishes the necessary condition for scalable metrological gain, while the sufficient condition requires the model to lie below the symmetry breaking transition. Therefore, in systems with random interaction graphs, the scaling of the spin-squeezing critical point emerges from a nontrivial interplay between xy-ferromagnetic universality and percolation universality. We apply this general theoretical framework to several experimental scenarios and discuss sharp and experimentally relevant conditions for achieving robust metrological gain on generic inhomogeneous structures, giving a unifying perspective for designing scalable quantum sensors across diverse quantum simulation platforms.
Dynamical susceptibility and quantum Fisher information in the Su-Schrieffer-Heeger model with Hatsugai-Kohmoto interactions
We investigate the dynamical spin and charge susceptibilities and the associated quantum Fisher information in a class of interacting lattice models, with a primary focus on the Su-Schrieffer-Heeger model in the presence of Hatsugai-Kohmoto interactions. To provide a rigorous analytical benchmark, we contrast the response properties of the SSH-HK system with those of the single-band Hubbard and SSH-Hubbard models, treated within the random-phase approximation. While standard Hubbard-type interactions typically suppress excitation strength, we demonstrate that the SSH-HK model displays qualitatively distinct physical behavior arising from the interplay between SSH dimerization and the momentum-diagonal nature of the HK interaction. Leveraging the exact solvability of the HK term, we derive closed-form expressions for the dynamical susceptibility, revealing unique filling-controlled characteristics such as a finite response at zero wave vector and a pronounced restructuring of spectral weight across integer and fractional filling sectors. We show that the quantum Fisher information, defined as the frequency integral of the imaginary part of the susceptibility, serves as an efficient probe of these filling sectors, exhibiting distinct piecewise behavior that distinguishes integer from fractional fillings. Notably, our results indicate that the quantum Fisher information remains insensitive to topological transitions within uniform-density regimes, highlighting the limitations of standard dynamical response functions in characterizing band topology. These findings establish the SSH-HK model as a powerful analytical platform for exploring the competition between topology and strong correlations, demonstrating how dynamical susceptibilities and the quantum Fisher information provide complementary, experimentally accessible probes of many-body physics.
On the Relation Between String Order Parameters, Entanglement, and Dynamical Quantum Phase Transitions in Topological Dynamics
That author's affiliation: Maria Curie-Skłodowska University First author institution: Raja Rammohun Roy Mahavidyalaya Last author institution: Maria Curie-Skłodowska University
Topological order is defined by topological invariants, rather than symmetries and local order parameters. Nonetheless some topological phases can be characterized by string order parameters and entanglement. In this article we study how string order parameters and entanglement spectra behave out-of-equilibrium following quenches in one dimensional topological models with $\mathbb{Z}$ invariants. Previously it has been suggested that string order parameters could serve as an experimental probe of dynamical quantum phase transitions. Despite the existence of clear zeroes in the order parameters at critical times, we show that in general there is no exact quantitative or qualitative connection with the critical times of dynamical quantum phase transitions. Another possible connection is of dynamical string order parameter zeroes and dynamical crossings at the center of entanglement spectra. Here we see that there can sometimes be a connection, but it is not typical. Again there is no general quantitative or qualitative connection. Each dynamical form of criticality behaves independently, though we do see that critical times tend to be of the same order of magnitude and give an argument for why this is the case. We also find that a string order parameter which labels one topological phase can undergo non-trivial dynamics even following a quench between \emph{other} topological phases. We elucidate where connections can be made, and where they result from a consideration of insufficiently general models. These results cast doubt on the idea of genuine dynamical phases following quenches in such models.
Native topological readout on qubit hardware: a Fibonacci-chain benchmark of measurement-compilation trade-offs
Recent demonstrations of non-Abelian braiding of graph vertices on noisy intermediate-scale quantum (NISQ) superconducting processor, and the experimental realization of topological order in general on various quantum hardware platforms necessitate an important question: when does a native (topological) fusion readout genuinely help for topological anyonic Hamiltonians implemented on NISQ hardware? We use the Fibonacci anyons chain as a concrete model for understanding the trade-off between measurement cost and compilation cost in that setting. The comparison is made against a simple grouped-Pauli baseline, and is scored by a covariance-aware mean-squared-error (MSE) of the full energy estimator. We based our benchmark on two different important classes of quantum circuits, namely Floquet time-evolved and variational quantum eigensolver quantum circuits, with the underlying Hamiltonian consisting of both braiding and fusion interaction. Our analysis found that there is not a uniform best method across both problems: the fusion readout method performed better on Floquet-type circuits on both the MSE and covariance-aware sampling variance, while the grouped Pauli method performed better on VQE on the MSE but worse on sampling variance. We derive scaling laws, and compute shot-budget crossover points, where one method is operationally favored above the other. The relevance of this work extends beyond Fibonacci chains to two-dimensional topological models compiled on superconducting and other qubit-native platforms, and can be used as a guide in answering the question of when one should measure in the native operator basis of the target physics, or when it is better to fall back on Pauli-basis reconstruction.
Raman Circular Dichroism and Quantum Geometry of Chiral Quantum Spin Liquids
We show that the quantum geometry of fractionalized spin excitations in Mott-insulating quantum spin liquids (QSL) gives rise to a finite Raman circular dichroism (RCD) signal. We demonstrate the equivalence between the Loudon-Fleury framework and the light-matter coupling approach for effective spinon bands. Using the latter, we derive an analytical decomposition of the RCD into different contributions of the quantum geometry. This reveals the sensitivity of the RCD to the underlying structure of the wave functions and the handedness of the excitations, rather than a nonzero Chern number of spinon excitations. To illustrate this, we apply our approach to two examples, the Kitaev honeycomb model in a magnetic field and a chiral $U(1)$ QSL on the triangular lattice, and discuss its experimental relevance for candidate materials.
A sine-square deformation approach to quantum critical points in one-dimensional systems
We propose a method to determine the quantum phase boundaries of one-dimensional systems using sine-square deformation (SSD). Based on the proposition, supported by several exactly solved cases though not proven in full generality, that "if a one-dimensional system is gapless, then the expectation value of any local observable in the ground state of the Hamiltonian with SSD exhibits translational symmetry in the thermodynamic limit," we determine the quantum critical point as the location where a local observable becomes site-independent, identified through finite-size scaling analysis. As case studies, we consider two models: the antiferromagnetic Ising chain in mixed transverse and longitudinal magnetic fields with nearest-neighbor and long-range interactions. We calculate the ground state of these Hamiltonians with SSD using the density-matrix renormalization-group algorithm and evaluate the local transverse magnetization. For the nearest-neighbor model, we show that the quantum critical point can be accurately estimated by our procedure with systems of up to 84 sites, or even smaller, in good agreement with results from the literature. For the long-range model, we find that the phase boundary between the antiferromagnetic and paramagnetic phases is slightly shifted relative to the nearest-neighbor case, leading to a reduced region of antiferromagnetic order. Moreover, we propose an experimental procedure to implement the antiferromagnetic $J_1$-$J_2$ Ising couplings with SSD using Rydberg atom arrays in optical tweezers, which can be achieved within a very good approximation. Because multiple independent scaling conditions naturally emerge, our approach enables precise determination of quantum critical points and possibly even the extraction of additional critical phenomena, such as critical exponents, from relatively small system sizes.
Emergent Spin Supersolids in Frustrated Quantum Materials
Recent years have witnessed the emergence of spin supersolids in frustrated quantum magnets, establishing a material-based platform for supersolidity beyond its original context in solid helium. A spin supersolid is characterized by the coexistence of longitudinal spin order that breaks lattice translational symmetry and transverse spin order associated with the spontaneous breaking of the spin U(1) symmetry. Extensive experimental investigations, together with advanced numerical studies, have now revealed a coherent and internally consistent picture of these phases, substantially deepening our understanding of supersolidity in quantum magnetic materials. Beyond their fundamental interest as exotic quantum states, potential applications in highly efficient demagnetization cooling have been supported by a giant magnetocaloric effect observed in candidate materials. Moreover, the possible dissipationless spin supercurrents could open promising perspectives for spin transport and spintronic applications. This review summarizes recent progress on emergent spin supersolids in frustrated triangular-lattice quantum antiferromagnets, surveys experimental evidence from thermodynamic and spectroscopic measurements, and compares these results with theoretical studies of minimal models addressing global phase diagrams, ground state properties, and collective excitations. In addition, this review discusses characteristic spin-transport phenomena and outlines future directions for exploring spin supersolids as functional quantum materials.
Emergent relativistic symmetry from interacting fermions on the honeycomb bilayer
We study the phase diagram of interacting spinless fermions on the honeycomb bilayer at charge neutrality using large-scale quantum Monte Carlo simulations. In the noninteracting limit, the low-energy spectrum features quadratically dispersing bands that touch at the corners of the hexagonal Brillouin zone. Weak to intermediate interactions induce a splitting of each of the quadratic band touching points into four Dirac points, located along high-symmetry directions of the reciprocal lattice. Strong interactions lead to the formation of a layer-polarized charge density wave, which spontaneously breaks the $\mathbb Z_2$ layer inversion symmetry and opens an insulating gap in the spectrum. We show that the semimetal-to-insulator quantum phase transition as a function of interaction is continuous and characterized by emergent relativistic symmetry. Our results for the values of the correlation-length exponent $\nu$, the order-parameter anomalous dimension $\eta_\phi$, and the fermion anomalous dimension $\eta_\psi$ agree with those of the theoretically predicted 2+1D Gross-Neveu-Ising universality class with eight two-component Dirac fermions within less than 5\%\ deviation. We also determine the crossover scale as a function of interaction strength between the nonrelativistic semimetal state at high temperatures, characterized by dynamical critical exponent $z = 2$, and the Dirac semimetal state at intermediates temperatures, characterized by $z=1$. Further reducing the temperature below the crossover scale at a fixed value of the interaction strength above the quantum critical point results in a classical ordering transition in the 2D Ising universality class.
Colossal Type-II Multiferroic Polarization Driven by Collinear Spin Orders
Achieving strong magnetoelectric coupling (MEC) together with large ferroelectric polarization remains a central challenge in type-II multiferroics. In conventional spin-driven multiferroics, the induced polarization is usually mediated by spin-orbit coupling (SOC) or spin-lattice coupling (SLC). Since many representative systems are based on 3d transition-metal ions, where SOC is relatively weak and SLC-induced lattice distortions are often limited, their polarizations are typically much smaller than those of proper ferroelectrics. Moreover, electric polarizations in type-II multiferroics are generally induced by spiral spin orders stabilized by competing magnetic interactions, which often leads to relatively low magnetic transition temperatures. In this Letter, using spin-group symmetry, we propose an SOC- and SLC-independent route to MEC in collinear 3d magnetic systems. We show that, even for a noncentrosymmetric lattice structure, different collinear magnetic configurations can either forbid or allow electric polarization, indicating direct magnetic control of polarization and hence strong MEC. The first-principles calculations excluding SOC on monolayer 2H-VS2 support this picture: a collinear stripy antiferromagnetic order induces an in-plane ferroelectric polarization up to 25.00 {\mu}C/cm2, about two orders of magnitude larger than that of typical type-II multiferroics. Furthermore, our microscopic model suggests that the induced polarization originates from SOC-independent p-d hybridization governed by electronic hopping. Our results suggest a possible route toward type-II multiferroics combining strong MEC with large electronic polarization in collinear 3d magnetic systems.
Effects of Band Symmetry on Spin-Dependent Transport in Noncollinear Antiferromagnetic Tunnel Junctions
Antiferromagnetic tunnel junctions (AFMTJs) can exhibit large tunneling magnetoresistance (TMR), making them promising candidates for ultrafast and field-robust spintronic devices. Here, we elucidate the role of band symmetry in governing spin-dependent transport in AFMTJs. Using first-principles density-functional theory combined with quantum-transport calculations, we investigate Mn3NiN/LaAlO3/Mn3NiN (001) junctions based on the noncollinear $\Gamma_{4g}$ antiferromagnetic phase of Mn3NiN. Although Mn3NiN exhibits a large momentum-dependent spin polarization due to broken $PT$ symmetry, we show that the tunneling conductance is critically controlled by band symmetry of the electrode Bloch states and their symmetry-selective coupling to evanescent states in the LaAlO3 barrier. Orbital-symmetry selection rules suppress interband transmission in the parallel configuration, whereas the antiparallel configuration enables symmetry-compatible interband tunneling along the diagonal directions of the two-dimensional Brillouin zone. These additional transmission channels enhance the antiparallel conductance and reduce the TMR relative to predictions based solely on spin polarization. Nevertheless, the TMR remains exceptionally large, exceeding 2000%, while band symmetry controls the attainable magnitude of TMR in AFMTJs. Our results establish band-symmetry filtering as an essential ingredient of spin-dependent tunneling in AFMTJs.
Electrically Controllable Flat Band in Two-Dimensional Electron Gases under Nonuniform Magnetic Fields
Flat bands underlie a diverse range of quantum phenomena, from strongly correlated phases to superconductivity. We theoretically establish that a two-dimensional electron gas under a linear magnetic-field gradient and a transverse electric field exhibits electrically tunable flat bands. At specific field values, these bands become strictly dispersionless. By providing exact classical and quantum solutions, we demonstrate that these states are high-order Landau levels associated with drift-compensated cyclotron orbits of carriers arising from the synergy between the magnetic-field gradient and the electric field. These electrically controllable Landau levels exhibit quantized Hall conductance and a strongly enhanced density of states. Our results provide a new route for flat-band creation, magnetoelectric band engineering, and quantized Hall currents controlled via source-drain voltage.
Emergence of Triplet Superconductivity from Cavity Vacuum Fluctuations
Engineering quantum materials with cavity fields has emerged as a powerful route to manipulate phases of quantum matter in solids. Here we demonstrate that cavity vacuum fluctuations alone can drive the emergence of triplet superconductivity in an otherwise singlet superconductor. The vacuum field renormalizes the electronic band structure in a polarization dependent manner, reshaping the Fermi surface and altering the competition among symmetry allowed pairing channels. As a result, multiple superconducting phases arise from the cavity vacuum fluctuations. Above a critical light matter coupling, the leading instability switches from singlet to triplet pairing, yielding a superconducting state absent in the bare material. This vacuum induced symmetry transition produces distinct modifications of the gap structure and low energy quasiparticle spectrum. Our results establish cavity vacuum engineering as a mechanism for generating unconventional superconducting phases and stabilizing triplet states of potential relevance for topological superconductivity.
Quasinormal mode quantization of bound and propagating photons in complex lightguiding nanostructures for integrated devices
Open optical or plasmonic resonators are placed on and connected through surfaces or via waveguides, forming complex lightguiding nanostructures, e.g. for integrated photonic quantum devices. We derive general boundary conditions for quasinormal modes that account for the structure's specific geometry. We then present a general quantization scheme for multiple, interacting quasinormal-mode cavities coupled to quantum emitters and to a non-bosonic bath of propagating photons on waveguides or a surface. We derive a system-bath Hamiltonian with rigorously defined coupling elements that can be computed using Maxwell solvers, including light-matter coupling between the electromagnetic field and quantum emitters. We define system-bath correlation functions for an effective, bath-mediated, and time-delayed interaction between the quasinormal modes and quantum emitters, which is a main ingredient commonly used to simulate open quantum system dynamics.
Topologically Driven Giant Effective Spin Mixing Conductance in Antiferromagnetic FeSn/Py Heterostructures
The topological semimetal FeSn antiferromagnet, characterized by its kagome lattice, two-dimensional flat bands, and Dirac-like surface states, holds immense promise for spintronic applications. In this work, for the first time, we investigate the spin pumping behavior in epitaxial-FeSn/Py (Ni$_{80}$Fe$_{20}$) heterostructures. We report a giant effective spin mixing conductance (g$^{\uparrow \downarrow}_{\mathrm{eff}}$) of $(116\pm 7)$~nm$^{-2}$, which is nearly one order of magnitude higher than that of standard Pt/Py heterostructures. The insertion of a 3 nm Al spacer layer results in a two-fold reduction in the effective damping, confirming the interfacial origin of the large g$^{\uparrow\downarrow}_{\mathrm{eff}}$. Consistently, we observe an order-of-magnitude higher inverse spin Hall effect voltage in the FeSn/Py system compared to a reference Pt/Py film stack. We attribute the giant g$^{\uparrow\downarrow}_{\mathrm{eff}}$ to the direct interfacing of the Py layer with the topologically active [001]-kagome surface of epitaxial-FeSn. These findings establish the critical role of topologically active interfaces for advanced quantum-material-based spintronic devices.
Quantum-metric Bloch oscillations in weakly inhomogeneous electric fields
Geometric analogs of Bloch oscillations studied so far have relied on Berry curvature. We show that a weakly inhomogeneous electric field adds a distinct quantum-metric term to semiclassical wavepacket dynamics, generating an oscillatory real-space contribution even when the Berry curvature vanishes. The associated transport response comprises an intrinsic and a scattering-time-dependent part. In the regime studied, the latter can dominate and approach finite saturation at high field when the relative field inhomogeneity is held fixed. A tilted Dirac model illustrates the mechanism. Realistic platforms will likely require synthetically engineered superlattices, with a finite quantum metric and an adequate band gap.
Topological semimetals: surface transport and spin effects
That author's affiliation: Osipyan Institute of Solid State Physics RAS Institution (first & last author): Osipyan Institute of Solid State Physics RAS
For the solid state physics, recent interest to topological systems is mostly connected with topological semimetals, in particular, to Weyl ones as the most representative semimetal type. Like other topological materials, e.g. topological and Chern insulators, topological semimetals acquire topologically protected surface states with linear dispersion. In contrast to helical surface states in topological insulators, the surface states are chiral for Weyl semimetals, similarly to Chern insulators, which allows to consider Weyl semimetals as the three-dimensional analog of the quantum Hall effect regime. Weyl semimetals are also interesting for spin-dependent effects, due to the spin-momentum locking in the topological surface states. For topological semimetals, the main problem of transport investigations is to reveal the surface states contribution in the material with gapless bulk spectrum. Here, we present review of experimental results on charge and spin transport in topological semimetals: charge transport in different superconducting proximity devices; spin-dependent transport; magnetic response of the topological surface states; non-linear anomalous Hall effect as the direct manifestation of the non-zero Berry curvature in topological semimetals. Possible applications are also considered for this new class of topological materials.
Signatures of the Quantum Geometric Dipole of Interlayer Excitons in Counterflow Conductivity
Collective excitations of many-body electron systems can carry internal structure, supporting novel quantum geometric and topological properties. Among these are a quantum geometric dipole (QGD), which for excitons have direct significance as an internal polarization. For interlayer excitons of a bilayer system, this represents an in-plane dipole moment, which can be used to drive them with in-plane electric fields. In this work, we consider counterflow electric currents associated with driven excitons in such a bilayer system as a probe of their QGD structure. As a simple but non-trivial example, we analyze a structure with a one-dimensional periodic potential in a strong perpendicular magnetic field. The resulting magnetoexciton bands host QGD structure that distinguishes it from the exciton QGD of a uniform system. To model exciton transport we adopt a Boltzmann approach that includes inter-band tunneling, allowing us to consider non-equilibrium momentum distributions that result from strong layer-antisymmetric driving fields. We show how linear response to a layer-symmetric component of the driving fields provide information about the QGD, and that the broad QGD structure of the exciton bands can be probed by the varying the layer-antisymmetric field. Our results demonstrate that counterflow conductivity serves as a tunable probe of the internal quantum geometric structure carried by the interlayer excitons, connecting transport to the quantum geometry of many-body excitations.
Exact and mean-field analysis of the role of Hubbard interactions on flux driven circular current in a quantum ring
We investigate circular current in both ordered and disordered Hubbard quantum rings threaded by magnetic flux, employing exact diagonalization and the Hartree-Fock mean-field approach within the tight-binding framework. The influence of on-site and extended Hubbard interactions, disorder, and electron filling on the persistent current is systematically analyzed. To construct the full many-body Hamiltonian, we introduce a linear table formalism, which, to our knowledge, has been rarely used in this context. In ordered rings, the current decreases monotonically with increasing on-site repulsion, while the impact of the extended interaction depends strongly on the filling factor. At low filling, stronger extended interaction suppresses the current, whereas near half-filling, it enhances the current up to a critical ratio, half of the on-site strength, before reducing it. Disorder significantly modifies these behaviors, notably enhancing the current at less than quarter-filling with increasing extended interaction. The localization properties of eigenstates, examined via the inverse participation ratio, further support the crucial roles of filling and the interplay between on-site and extended interactions in governing persistent current.
Coupled-wire descriptions of unconventional quantum states in twisted nanostructures
Coupled-wire description has been developed as a powerful framework for providing bosonic descriptions of strongly correlated quantum matter, with early applications to systems such as the cuprates and the integer and fractional quantum Hall states. In this topical review, we discuss recent developments of coupled-wire description in nanoscale systems, where it emerges not only as a theoretical tool but also as a highly tunable physical platform. In these nanoscale realizations, coupled-wire networks are formed by one-dimensional channels embedded in two-dimensional materials, most prominently in moir\'e and twisted structures. Such networks host a broad range of unconventional states of matter, including superconductivity, charge density waves, spin density waves, Mott insulating phases, Anderson insulating phases, quantum spin Hall states, quantum anomalous Hall states, and their fractionalized counterparts. The ability to electrically control interaction strength, confinement, and coupling between wires makes these systems qualitatively different from earlier realizations and allows continuous tuning between competing phases. Notably, recent work has demonstrated that the coupled-wire framework in moir\'e networks completes the trio of quantum Hall phenomena, encompassing quantum Hall, quantum spin Hall, and quantum anomalous Hall states, together with their fractional analogues. This development highlights coupled-wire networks in nanoscale materials as a versatile and experimentally relevant setting for exploring the interplay of topology, strong correlations, and low-dimensional physics.
Probing persistent spin textures through nonlinear magnetotransport
Persistent spin textures (PST) are special spin configurations in spin-orbit-coupled systems in which the spin polarization acquires a symmetry-enforced momentum-independent orientation, leading to exceptionally long spin lifetimes and persistent spin helices. Identifying direct experimental probes of PST, however, remains challenging because conventional quantum-geometric responses are strongly suppressed in this regime. Here, we show that PST systems isolate spin-rotation quantum geometry, which manifests through distinctive nonlinear magnetotransport responses. Using both a fine-tuned Rashba-Dresselhaus two-dimensional electron gas and a symmetry-enforced cubic spin-splitting model realizing PST, we demonstrate that PST suppresses conventional and Zeeman quantum-geometric contributions, leaving the spin-rotation quantum geometric tensor as the sole source of nonlinear magnetic-current and spin-magnetization responses. Remarkably, the nonvanishing response components exhibit identical direction-independent behavior as a function of chemical potential, providing a distinctive signature of PST. We further show that, in the Rashba-Dresselhaus two-dimensional electron gas at the PST point, these qualitative signatures remain robust even in the presence of a cubic Dresselhaus term that breaks the exact SU(2) symmetry. Our results establish nonlinear magnetotransport as an experimentally accessible probe of PST and their underlying spin-rotation quantum geometry.
A textured polar phase in strained SrTiO3
Quantum materials can harbour hidden phases whose microscopic structures differ from conventional ordered states while reproducing their macroscopic signatures, making them easy to miss. Strontium titanate is a longstanding puzzle of this kind: on cooling it shows every hallmark of an incipient ferroelectric, yet never orders, and is usually described as a quantum paraelectric in which fluctuations suppress ferroelectricity. Here we combine uniaxial strain, single-cycle terahertz excitation and femtosecond x-ray scattering to measure the polar collective modes of strontium titanate as a function of momentum and strain. Under modest tensile strain, we observe a new vibrational mode that emerges not at the Brillouin zone centre, as a ferroelectric transition would require, but at finite wavevector, identifying the ordered state as a polar texture on nanometre length scales rather than a uniform ferroelectric. Unstrained quantum paraelectric strontium titanate is then naturally understood as the disordered precursor of this textured phase, offering a resolution to a decades-old puzzle and illustrating how finite-momentum collective excitations can unmask hidden phases in quantum materials.
Large-flavor route to a stable U(1) Dirac spin liquid on the maple-leaf lattice
The $\mathrm{U}(1)$ Dirac spin liquid provides a useful organizing framework for frustrated magnets: it offers an algebraic parent state from which competing orders, confinement patterns, and low-energy spectral features can be understood. Whether such a state can occur as a stable ground state of a two-dimensional spin Hamiltonian remains an open question, because monopole events of the compact gauge field can proliferate and confine the spinons. Here, we show that the maple-leaf lattice provides a distinct route to this problem. Its Dirac spin liquid realizes QED$_3$ with $N_f=12$ Dirac fermions, substantially more than the $N_f=4$ theories of the triangular and kagome lattices. We classify the fundamental monopoles under the full microscopic symmetry group and find five charge-one spin-singlet monopoles that are trivial under lattice symmetries, time reversal, and spin rotation. The phase is therefore not protected by symmetry in the usual sense: its stability depends on whether these allowed monopoles are dynamically irrelevant. Available large-$N_f$ and Monte Carlo estimates place the charge-one monopole dimension close to the relevance threshold in $(2+1)$ dimensions, making the maple-leaf lattice a concrete large-flavor platform for testing the stability of compact QED$_3$ in a quantum magnet. The same monopole classification gives direct numerical predictions, identifying the symmetry sectors in which singlet, triplet, and quintet monopole excitations should appear. This provides a route to testing the $N_f=12$ Dirac spin liquid through symmetry-resolved exact diagonalization and variational studies of maple-leaf spin Hamiltonians.
Observation of magnetically switchable quantum geometric photocurrents
In non-centrosymmetric materials, light can be rectified into two types of DC photocurrents, known as injection and shift currents, through the bulk photovoltaic effect. Recent theory has uncovered their deep relation with the two-state quantum geometry of resonant transitions: In non-magnetic crystals, where these currents have been routinely observed, the injection current responds to circular light and probes the Berry curvature, while the shift current responds to linear light and probes the geometric connection. Magnetic crystals have been predicted to show a new set of hitherto unobserved magnetically switchable photocurrents, with the roles of linear and circular light interchanged: A linear injection current, which probes the quantum metric, and a circular shift current, which probes the geometric torsion. In this work, we demonstrate the existence of such currents for the first time, demonstrating the switching of the current by flipping the N\'eel vector in a van der Waals antiferromagnet. Furthermore, their specific frequency and temperature dependence confirm the assignment of circular shift and linear injection currents. Our work demonstrates a new way to control photocurrents in magnets that are directly tied to geometry and have promising applications in antiferromagnetic spintronics and light harvesting.
Optical control of conductivity type and valley polarization via persistent photoconductivity in (Pb,Sn)Se quantum wells
That author's affiliation: Johannes Kepler University of Linz Institution (first & last author): Institute of Physics
The ability to tune the Fermi level of semiconductors is at the heart of modern electronics. Here, we demonstrate that persistent photoconductivity (PPC) enables tuning of carrier density, conductivity type, and, consequently, the valley polarization in (Pb,Sn)Se/(Pb,Eu)Se quantum wells. Illumination of these samples induces Fermi level shifts that convert the system from a threefold-degenerate $\bar{M}$-valley two-dimensional hole gas to a single $\bar{\Gamma}$-valley-polarized electron gas with similar values of mobility. The optically induced state persists for more than $10^{3}$ minutes at cryogenic temperatures and enables stepwise optical gating without the need for device processing. These transitions are confirmed by the sign inversion of the Hall slope and the modification of quantum Hall plateau degeneracies measured in magnetic fields up to 35 T. Landau level $k\cdot p$ model calculations quantitatively reproduce the experimental data. Furthermore, studies of weak-field magnetoresistance demonstrate the significance of quantum localization phenomena at the transition between the weakly and strongly localized regimes in compensated narrow-gap semiconductors. Spectral studies allow us to identify the critical role of the barrier material and determine the photon energies that can reverse the PPC effect. The persistent light-induced upward shift of the Fermi level in the $p$-type quantum well is explained in terms of specific energy positions of donor and acceptor defect states in the studied system. Our results demonstrate that PPC is a powerful optical gating tool for the IV-VI quantum wells, a versatile platform for reconfigurable valleytronic architectures.
Harnessing hidden quantum metric response in a 2D magnet via nonlocal photovoltaic effect
The quantum geometry of Bloch wavefunctions underpins a wealth of emergent phenomena in quantum materials. Its imaginary part, the Berry curvature, has long been recognized as a key source for hallmark effects such as quantum Hall and topological phenomena, etc. The real part of quantum geometry, the quantum metric, has recently garnered considerable attention due to predictions of a range of unconventional nonlinear and nonequilibrium responses. Such responses usually vanish in centrosymmetric systems, largely restricting relevant studies to non-centrosymmetric materials. Here we challenge this convention by revealing that the vanished quantum metric response can survive in a hidden form. Using a non-local photovoltaic scheme in a layered magnetic semiconductor, we spatially separate mutually compensating photocurrents and thereby detect such hidden quantum metric response. We demonstrate this effect across distinct magnetic states and down to the ultrathin limit. Moreover, we realize reconfigurable, nonvolatile and probabilistic photodetection enabled by the quantum metric response. These results not only fundamentally expand the material landscape for quantum geometric physics, but also open new gateway to harvest the quantum geometric contributions for state-of-the-art nonvolatile reprogrammable sensing and computing applications.
Non-Bloch Quantum Geometry of Non-Hermitian Systems
We formulate quantum geometry for non-Hermitian systems under open boundary conditions. By defining quantum-geometric quantities in both real-space and non-Bloch representations, we establish a unified framework beyond conventional Bloch band theory. Our central result is an exact equivalence between the real-space integrated quantum metric and a non-Bloch integrated quantum metric defined on the generalized Brillouin zone. We further introduce localized non-Bloch Wannier functions in the presence of the non-Hermitian skin effect and show that the non-Bloch integrated quantum metric gives the gauge-invariant part of their spread functional. These results establish quantum geometry as a natural framework for characterizing open-boundary non-Hermitian band structures and the localization properties encoded in skin modes.
Twisted light generates robust many-body states for practical quantum computing
That author's affiliation: Universidad de Los Andes First author institution: Universidad de Los Andes Last author institution: George Washington University
Twisted light carries orbital angular momentum (OAM) and can drive excitations of confined, interacting electrons that are dark to uniform dipolar probes. Here we show how this ``beyond-Kohn's-Theorem'' optical channel can become a concrete control primitive for quantum computing. Correlation sectors in few-electron quantum dots -- characterized by the relative angular momentum quantum number -- form a tunable ladder of many-body states that are robust in the limited sense of symmetry-protected selection rules and persistent chiral spectroscopic fingerprints; full topological gap protection requires three or more electrons. A twisted-light pulse with prescribed OAM index and polarization provides fast optical write, read, and scalable addressing of these sectors via the selection rule $\Delta|m|=\pm(l+\sigma)$. In the analytically solvable Calogero ($1/r^2$) interaction limit, both the energy spectrum and the twisted-light matrix elements are closed-form functions of the interaction strength, allowing gate parameters (Rabi frequency, qubit frequency, anharmonicity, and leakage rates) to be written down explicitly. We map these results onto a universal single-qubit gate set, propose a concrete two-qubit entangling mechanism via state-dependent Coulomb coupling between adjacent dots, and identify the dominant decoherence channel (quadrupolar charge noise). A semi-analytic $N=3$ extension using the $1/N$ expansion provides a design-level scaffold for the topological roadmap, including quasihole sector addressing. The central operational message is that twisted light enables WRITE (pulse-create a correlation sector), READ (spectroscopically diagnose correlations), and SCALE (optical addressing via spatial light modulator) in a unified photonic control layer. Throughout, screened and Coulomb interactions preserve the same qualitative chiral fingerprints established in the solvable limit.
Spectral and transmission properties of multiple correlated quantum dots made simple
That author's affiliation: University of the Basque Country First author institution: The Abdus Salam International Centre for Theoretical Physics (ICTP) Last author institution: University of the Basque Country
Steady-state density functional theory, called i-DFT, is employed to compute spectral and transmission properties of general interacting nanoscale regions coupled to electronic reservoirs. Exchange-correlation functionals are constructed for different interactions and coupling geometries. The potential of the method is illustrated by applications to various multiple quantum dots from the Coulomb blockade to the Kondo regime, capturing phenomena such as quantum phase transitions. The results are in excellent agreement with many-body approaches at a fraction of the computational cost.
Towards complete characterization of topological insulators and superconductors: A systematic construction of topological invariants based on Atiyah-Hirzebruch spectral sequence
The past decade has witnessed significant progress in topological materials investigation. Symmetry-indicator theory and topological quantum chemistry provide an efficient scheme to diagnose topological phases from only partial information of wave functions without full knowledge of topological invariants, which has resulted in a recent comprehensive materials search. However, not all topological phases can be captured by this framework, and topological invariants are needed for a more refined diagnosis of topological phases. In this study, we present a systematic framework to construct topological invariants for a large part of symmetry classes, which should be contrasted with the existing invariants discovered through one-by-one approaches. Our method is based on the recently developed Atiyah-Hirzebruch spectral sequence in momentum space. As a demonstration, we construct topological invariants for time-reversal symmetric spinful superconductors with conventional pairing symmetries of all space groups, for which symmetry indicators are silent. We also validate that the obtained quantities work as topological invariants by computing them for randomly generated symmetric Hamiltonians. Remarkably, the constructed topological invariants completely characterize $K$-groups in 159 space groups. Our topological invariants for normal conducting phases are defined under some gauge conditions. To facilitate efficient numerical simulations, we discuss how to derive gauge-independent topological invariants from the gauge-fixed topological invariants through some examples. Combined with first-principles calculations, our results will help us discover topological materials that could be used in next-generation devices and pave the way for a more comprehensive topological materials database.
Single excitation swap in a modified Jaynes-Cummings-Hubbard lattice
Controlling the transport and nature of quantum excitations in low-dimensional systems is a key requirement for scalable quantum devices, including communication networks and quantum simulators. We propose a one-dimensional hybrid quantum lattice model, in which each lattice unit integrates a single-mode resonator that interacts with a two-level system (TLS), featuring direct coupling between adjacent TLSs. This configuration enables the coherent propagation of excitations with tunable atomic, photonic, or polaritonic character. Beyond conventional single-excitation transport, we demonstrate that appropriate impedance-matching and resonance conditions allow for the controlled swapping of excitation type as the excitation propagates along the lattice. We analyze the resulting dynamics using local observables and pairwise concurrence to track both transport and quantum correlations. Our results establish a minimal platform for controlled single-excitation conversion, with direct relevance to hybrid quantum networks, on-chip quantum interconnects, and engineered quantum simulators.
$d$-wave Surface Altermagnetism in Centrosymmetric Collinear Antiferromagnets
Broken inversion symmetry at the surfaces of centrosymmetric collinear antiferromagnets lifts combined inversion and time-reversal symmetry ($PT$) and can, in principle, enable nonrelativistic d-wave spin splitting, termed surface altermagnetism. Combining symmetry analysis with first-principles calculations, we show that surface inversion breaking, while necessary, is not sufficient for this effect. Surface altermagnetism emerges only when no antiunitary symmetry survives at the surface that exchanges the two antiferromagnetically coupled surface sublattices and enforces spin degeneracy. We demonstrate this mechanism explicitly for the centrosymmetric G-type antiferromagnets V$_3$Al and BaMn$_2$Sb$_2$, and contrast it with MnPt, where a sublattice-exchanging symmetry survives at the surface in the form of translation-time-reversal symmetry ($tT$), thereby preserving spin degeneracy despite broken inversion symmetry. The mechanism is shown to apply across multiple classes of centrosymmetric antiferromagnets and remains robust against spin-orbit coupling, although relativistic spin mixing in heavier-element compounds may reduce the observable spin polarization. These results establish a symmetry-based route toward realizing robust nonrelativistic momentum-dependent spin polarization at antiferromagnetic surfaces and interfaces.
Deconfined Boundary Phase Transition of a Quantum Critical Heisenberg Model
We investigate the boundary phases of a (2+1)-dimensional quantum critical Heisenberg model with a dangling spin chain. By introducing a multispin $Q$-term along the boundary, we drive a continuous boundary transition from an antiferromagnetic (AF) order to a valence-bond solid (VBS) order. Using large-scale quantum Monte Carlo simulations, we locate the critical point at $Q_{c}=0.310(11)$, and obtain the critical exponents at $Q_{c}$, including $y_{s}=0.81(4)$ and the scaling dimensions of AF and VBS order parameters $\Delta_{s}=0.660(15)$ and $\Delta_{v}=0.204(14)$. The weak long-range AF order for $Q<Q_{c}$ is stabilized by quasi-long-range effective interactions mediated by the critical bulk state, while the VBS phase restores the ordinary critical behavior. Our findings highlight the synergy between topological terms and quasi-long-range interactions in low-dimensional quantum many-body systems.
Geometric curvature driven by many-body collective fluctuations
Quantum geometry characterizes the variation of wavefunctions in momentum space through their overlaps and relative phases, providing a general framework for understanding many transport and optical properties. It is generally formulated in terms of interband matrix elements, which, entering the response functions, allow obtaining experimental access to the quantum geometric tensor. Recently, it has been emphasized that quantum geometry can also be interpreted in terms of quantum dipole fluctuations in the ground state driven by interband mixing. Here, we extend this picture to include contributions from many-body collective fluctuations, in which propagators and response vertices are dressed dynamically by the interaction with collective modes. Focusing on the Berry curvature, we show that contributions from collective fluctuations can be experimentally distinguished from bare band-geometric contributions, via specific antisymmetric channels in inelastic scattering spectra. We further identify the non-commutative properties of transverse quantum fluctuations as well as non-local-time interactions as the generators of this dynamical curvature in the susceptibility response.
Finite-temperature spin diffusion in the two-dimensional XY model
We present a combined theory-experiment study to quantify spin diffusion in the square lattice quantum spin-1/2 XY model at finite temperature. On the theory side, we leverage a recently developed dynamical high-temperature expansion method to faithfully capture the long spatiotemporal scales of the hydrodynamic regime. Experimental results are obtained from an optical lattice hard-core boson quantum simulator. The excellent agreement of spin diffusion constants marks a breakthrough in spin-transport beyond one dimension and for the quantitative validation of state-of-the-art quantum simulation platforms. We also provide theory predictions for future experiments on dynamic spin conductivity or anisotropy-induced integrability breaking.
Quantum-Critical, Spin-Fluctuation-driven Residual Resistivity and Emergent Universal Correlations in the Fermi-Liquid Regime of Heavy-Fermion Superconductors
We investigate correlations within the unconventional Fermi-liquid (FL) regime of quantum-critical (QC) heavy-fermion superconductors (HFSs) by tracking the pressure dependence of three quantities: the temperature-independent, SF-driven residual resistivity, $\rho^{ sf}_{0}(P)$; the FL scattering coefficient, $A(P)$; and the superconducting transition temperature, $T_c(P)$. The first two define the spin-fluctuation contribution to the resistivity, $\rho(T)=\rho^{sf}_0+AT^2$. Using experimental data from archetypal heavy-fermion systems, we identify three robust empirical correlations: $\ln(\frac{T_c}{\theta}) \propto A^{-1/2}$, $A \propto (\rho^{sf}_0)^2$, and $\ln(\frac{T_c}{\theta}) \propto \big(\rho^{sf}_0\big)^{-1}$ ($\theta$ is a characteristic temperature scale). Absent in conventional FL superconductors, these relationships indicate that QC fluctuations not only mediate inelastic scattering and Cooper pairing, but also generate an effective elastic channel responsible for $\rho^{sf}_0$. We explicitly calculate $\rho^{sf}_0$ on the high-pressure side of the quantum critical point (QCP) and introduce a characteristic length scale, $\ell \sim \big(\rho^{sf}_0\big)^{-1}$, that captures the spatial extent of fluctuation-induced scattering. Within this regime, and within the Migdal--Eliashberg framework combined with Boltzmann transport theory, we derive analytic expressions for $T_c(\ell)$ and $A(\ell)$, together with their interrelations, which are consistent with the observed empirical trends. These findings highlight the quantum-critical FL regime in HFSs as an intrinsically correlated phase, governed by fluctuations and marked by unconventional transport and pairing mechanisms.
Topology of the Fermi surface and universality of the metal-metal and metal-insulator transitions: $d$-dimensional Hatsugai-Kohmoto model as an example
The earlier theory [1] of the quantum phase transitions related to the change of the Fermi Surface Topology (FST) is advanced. For such transitions the Fermi surface as a quantum critical manifold determined by the Lee-Yang zeros, the order parameter $\mathcal{P}$ as the $d$-volume of the Fermi sea, and the special FST universality class were introduced in [1]. The exactly solvable Hatsugai-Kohmoto (HK) $d$-dimensional ($d=1,2,3$) model of interacting fermions is analyzed. We explore the relation between the Lee-Yang zeros, the Luttinger and the plateau (Oshikawa) theorems. The validity of the Luttinger theorem in the HK model is confirmed. It is shown that the order parameter $\mathcal{P}$ and the FST universality class describe the transitions between metal and band/Mott insulators, as well as the Lifshitz and van Hove gapless-to-gapless transitions. The gapless phases are established to be the Landau Fermi liquids (metals). In addition to the conventional paradigm with a continuous order parameter, we apply the homology theory to analyze the FST transitions. They are critical points of the Morse function. To quantify FST we use the Euler characteristic, which is calculated for each phase of the HK model. We claim that the FST universality class is robust with respect to interactions and other model details, under the condition that the critical points are non-degenerate.
Quantum-Coherent Regime of Programmable Dipolar Spin Ice
Frustrated spin-ice systems support emergent gauge fields and fractionalized quasiparticles that act as magnetic monopoles. Although artificial platforms have enabled their direct visualization, access to their quantum-coherent dynamics has remained limited. Here we realize a programmable dipolar square spin-ice model using a superconducting-qubit quantum annealer, providing access to a previously unexplored quantum-coherent regime of artificial spin ice. By implementing a direct one-to-one mapping between lattice spins and physical qubits, together with engineered extended couplings, we realize effective dipolar interactions on frustrated lattices comprising more than 400 vertices. Tuning transverse-field fluctuations enables us to probe the real-time dynamics of Dirac-string defects and interacting monopole plasmas. We observe super-diffusive monopole transport, with scaling exponents intermediate between classical diffusion and ballistic motion, indicating dynamics beyond classical stochastic relaxation and consistent with coherent propagation within an emergent gauge manifold. These results establish programmable quantum spin ice as a scalable platform for investigating fractionalized excitations and emergent gauge dynamics in engineered quantum matter.
Staggered spin susceptibility at a two-dimensional antiferromagnetic quantum critical point
We report on the finite temperature staggered spin susceptibility $\chi(Q)$ as a function of the mode-mode coupling constant $y_1$ in the self-consistent renormalization theory of two-dimensional antiferromagnetic spin fluctuations with zero-point quantum fluctuations just at the quantum critical point ($y_0$ = 0). We find that the value $y_1$ = 0.1 is a criterion to classify the effect of the zero-point spin fluctuations on the temperature dependence of $\chi(Q)$ into a Curie law for weak $y_1 < $ 0.1 and a Curie-Weiss type or a power law type for strong $y_1 > $ 0.1.
Efficient Quantum Implementation of Dynamical Mean Field Theory for Correlated Materials
That author's affiliation: CRD - Computational Research Division [LBNL Berkeley] (United States) Institution (first & last author): North Carolina State University
The accurate theoretical description of materials with strongly correlated electrons is a formidable challenge in condensed matter physics and computational chemistry. Dynamical Mean Field Theory (DMFT) is a successful approach that predicts behaviors of such systems by incorporating some of the correlated behavior using an impurity model, but it is limited by the need to calculate the impurity Green's function. This work proposes a framework for DMFT calculations on quantum computers, focusing on near-term applications. It leverages the structure of the impurity problem, combining a low-rank Gaussian subspace representation of the ground state and a compressed, short-depth quantum circuit that joins state preparation with time evolution to compute Green's functions. We demonstrate the convergence of the DMFT algorithm using the Gaussian subspace in a noise-free setting, and show the hardware viability of circuit compression by extracting the impurity Green's function on IBM quantum processors for a single impurity coupled to three bath orbitals (8 qubits, 1 ancilla). We discuss potential paths toward realizing this quantum computing use case in materials science.
Deep Spin Defects in Zinc Oxide for High-Fidelity Single-Shot Readout
Wide-bandgap oxides such as ZnO are favorable hosts for spin defect qubits due to their dilute nuclear spin background and potential for ultra-high purity. Yet, a deep-level defect qubit with robust optical and spin properties has not been identified in this material. Here, using first-principles calculations, we predict that the molybdenum-vacancy complex, Mo_Zn-V_O, exhibits the essential characteristics of an optically addressable spin qubit: a spin-triplet ground state, visible-range optical transitions with high quantum yield, and an unusually small Huang-Rhys factor (~5, compared to 10-30 in known ZnO defects). We further find long spin coherence times (T_2 ~ 4 ms) when both nuclear and impurity spin baths are considered, with paramagnetic impurities setting a threshold concentration of 0.035 ppm. Importantly, the combination of strong spin-orbit coupling and the absence of Jahn-Teller distortion supports spin-selective intersystem crossing and high-fidelity single-shot readout at elevated temperatures and across wide magnetic field ranges. By identifying ZnO as a host for deep-level defect qubits, our work points toward a pathway to scalable, integrable oxide-based quantum technologies and broadens the material foundation for solid-state quantum information science.
Quantum effective action for dissipative semiclassical dynamics
Using the quantum effective action in the Schwinger-Keldysh formalism, we derive quantum corrections to the semiclassical Langevin dynamics of a dissipative system governed by a macroscopic degree of freedom. We discuss the connection with the Ehrenfest theorem and show that, in the low-temperature and weak-damping regime, quantum corrections are determined by the zero-point energy of fluctuations evaluated at the classical underdamped frequency, closely paralleling the conservative case. We apply these general results to the resistively and capacitively shunted superconducting Josephson junction and to an elongated bosonic junction, where quantum corrections can reach the percent level under realistic conditions.
Entropy Production from Spin--Vibrational Coupling in Endohedral-Fullerene Qubits Encapsulated in Suspended Carbon Nanotubes
Hybrid carbon nanotube-fullerene architectures provide a controllable platform for studying irreversibility and information flow in structured quantum environments. We analyze entropy generation in a system where paramagnetic endohedral fullerenes, such as N@C$_{60}$ and P@C$_{60}$, are encapsulated inside a suspended carbon nanotube (CNT) resonator, with selected multi-level fullerene spin states forming an effective qubit coupled to quantized CNT flexural modes. Building on prior work on fullerene-filled CNTs, spin-phonon control in suspended nanotubes, and phase-space propagators for damped driven oscillators, we develop a hybrid open-system model combining driven quantum Brownian motion of the CNT with an effective Jaynes-Cummings spin-vibrational interaction. The resonator dynamics are represented by a Wigner function whose evolution is written analytically in terms of the initial Wigner distribution and a Gaussian propagator. This phase-space description separates drive-induced displacement, diffusion, and damping, and connects these processes directly to entropy flow. The coupled spin-mechanical dynamics are embedded in a Lindblad master equation including mechanical damping, spin relaxation, pure dephasing, and thermally activated excitation. Within this framework we derive the entropy balance, identify entropy flux and non-negative entropy production, and examine how spin-vibrational hybridization redistributes irreversibility between coherent exchange and dissipative channels. We show that magnetic-gradient-enhanced spin-phonon coupling, resonant driving, and moderate thermal occupation produce crossovers between oscillator-dominated and spin-dominated entropy-production regimes. The framework provides a basis for using CNT-PEF hybrids as nanoscale platforms to study nonequilibrium quantum thermodynamics, decoherence, and information loss in vibrational environments.
Quantum Geometry-Driven Nonlinear Spin Currents in Floquet Non-Hermitian Altermagnets
Altermagnets are rapidly emerging as a highly promising platform for spintronics, yet dynamically controlling their spin responses remains a fundamental challenge. In this work, we demonstrate that introducing periodic optical driving and non-Hermiticity provides a powerful route to achieve tunable control over these systems. We derive a general analytical expression for nonlinear spin currents in non-Hermitian phases with a spectral line gap, revealing that the intrinsic response cleanly separates into quantum metric, Berry curvature, and Berry connection dipole contributions. Applying this formalism to a Floquet non-Hermitian $d$-wave altermagnet, we uncover that the nonlinear spin conductivity is overwhelmingly dominated by the bare quantum metric. Furthermore, we show that the optical field's polarization can actively tune -- and even strictly reverse -- the direction of both longitudinal and transverse spin currents. Our work establishes a quantum geometric framework for the optical manipulation of nonlinear spin transport in advanced magnetic materials.
Tunable Crossed Andreev Reflection in Bipolar Magnetic Semiconductors
Crossed Andreev reflection (CAR) is a nonlocal quantum transport phenomenon that arises at the interface between a superconductor and two spatially separated metals. In this process, an electron incident from one metal combines with another electron originating from the other metal to form a Cooper pair in the superconductor. As a consequence, a hole is emitted into the second metal, establishing a nonlocal electron-hole conversion process. In contrast to local Andreev reflection -- where electron-to-hole conversion occurs within the same region -- CAR intrinsically links two spatially separated carriers, giving rise to nonlocal correlations and quantum entanglement. In bipolar magnetic semiconductors (BMSs), the conduction and valence bands possess opposite spin polarizations. We propose to achieve tunable control of CAR by independently adjusting the chemical potentials of the two regions. By engineering the alignment of spin-polarized bands in the two BMS leads, CAR can be selectively enhanced or suppressed. This tunability enables precise manipulation of nonlocal transport, and correlated electron dynamics, offering promising prospects for spintronic and superconducting device applications.
Orbital Angular Momentum Textures and Currents in a Discrete Helix: Equilibrium and Linear Response
Recently, nonequilibrium orbital angular momentum in low-dimensional systems has attracted renewed attention. Here we introduce a minimal three-orbital tight-binding model for a single helical chain and show that chirality alone generates a momentum-dependent orbital-angular-momentum texture through Slater--Koster hybridization in the local basis $(p_r,p_\phi,p_z)$, without requiring atomic spin--orbit coupling. In the single-helix geometry, the radial orbital texture vanishes identically, while the azimuthal and longitudinal components remain finite and arise from the odd-in-momentum $(p_z,p_r)$ and $(p_r,p_\phi)$ sectors. As a result, the equilibrium average orbital texture vanishes by parity, although persistent-like orbital angular momentum currents may still exist and imply chirality-dependent end magnetization in a finite helix. Under an applied longitudinal electric field, the system develops a finite orbital Edelstein response, whereas the projected longitudinal orbital-current conductivity vanishes in the linear regime by parity. When spin degrees of freedom are included, the orbital texture acts as a source of spin polarization through orbital-to-spin transduction. The resulting spin response is controlled by orbital overlap scales much larger than the bare relativistic spin--orbit scale, making it a stronger candidate for spin injection than the conventional spin Edelstein mechanism. These results identify chirality as the minimal microscopic ingredient for generating orbital angular momentum response in one-dimensional systems and support an orbital route to spin selectivity in chiral conductors.
Reversible nanoscale patterning of WTe$_2$ with a scanning tunneling microscope
Manipulating the lattice structure of ferroelectric quantum materials enables their use in low-power electronic devices, including field-effect transistors. WTe$_2$ is a Weyl-semimetal candidate and ferroelectric, both properties arising from the reduced crystal symmetry of its T$_\mathrm{d}$ ground state. The T$_\mathrm{d}$ crystal phase results from a Peierls distortion of the 1T parent structure and an interlayer shift. While experiments in WTe$_2$ have established ferroelectric switching and transient control of the predicted topological phase via ultrafast excitations, persistent electronic changes on the nanometer scale remain elusive. Here, we demonstrate that current pulses applied via scanning tunneling microscopy can both write and erase persistent nanometer-scale patterns on the surface of WTe$_2$. These patterns consist of apparent picometer in-plane and out-of-plane atomic displacements, accompanied by changes to the local density of states. The out-of-plane displacements further modulate the Peierls-like distortion present in WTe$_2$, while the in-plane displacements are indicative of ferroelectric switching. The induced patterns can be repositioned and erased, suggesting a nanoscale handle on the ferroelectric properties of WTe$_2$.
Interface Piezoelectric Loss in Superconducting Qubits
That author's affiliation: Lawrence Berkeley National Laboratory Institution (first & last author): Lawrence Berkeley National Laboratory
Dissipation remains a central obstacle to improving superconducting quantum circuits, yet the microscopic origins of loss in widely used materials platforms are not fully understood. Here, we report the observation of interface piezoelectricity-induced dissipation in superconducting qubits fabricated on high-resistivity silicon. Our devices use a transmon qubit with a shunt capacitor that simultaneously serves as an interdigital transducer embedded in a surface acoustic wave resonator. By tuning the qubit transition into resonance with discrete mechanical modes, we observe up to a factor-of-two reduction in qubit lifetime, consistent with energy exchange between the qubit and mechanical modes mediated by piezoelectric coupling at the aluminum-silicon interface. Our findings provide direct evidence for interface piezoelectricity as a distinct loss channel in superconducting qubits. Combined with multiphysics simulations, these findings suggest that interface piezoelectric loss can dominate over loss from two-level systems at sufficiently high frequencies.
Lieb-Schultz-Mattis constraints for hyperbolic lattices
The Lieb-Schultz-Mattis (LSM) theorem and its higher-dimensional extensions forbid the existence of a unique, symmetric, and gapped ground state at fractional fillings in quantum many-body systems with a conserved particle number (or spin angular momentum) and the conventional translation symmetry of Euclidean lattices. In this work, we propose a generalization of the LSM theorem to quantum many-body systems on hyperbolic lattices, i.e., regular tessellations of two-dimensional negatively curved space. By leveraging concepts from hyperbolic band theory in a many-body setting, we adapt Oshikawa's flux-threading argument to periodic hyperbolic lattices with a non-Euclidean (Fuchsian) translation symmetry and compute a lower-bound to the ground-state degeneracy as a function of filling and lattice geometry. We explore the consequences of LSM constraints for gapped phases of hyperbolic quantum matter and suggest frustrated spin models on hyperbolic analogs of the square and triangular lattices as promising platforms for realizing symmetric spin liquids in hyperbolic space.
The effects of alloy disorder on strongly-driven flopping mode qubits in Si/SiGe
In Si quantum dot systems, large magnetic field gradients are needed to implement spin rotations via electric dipole spin resonance (EDSR). By increasing the effective electron dipole, flopping mode qubits can provide faster gates with smaller field gradients. Moreover, operating in the strong-driving limit can reduce their sensitivity to charge noise. However, alloy disorder in Si/SiGe heterostructures randomizes the valley energy splitting and the valley phase difference between dots, enhancing the probably of valley excitations while tunneling between the dots, and opening a leakage channel. In this work, we analyze the performance of flopping mode spin qubits in the presence of charge noise and alloy disorder, and we optimize these qubits for a variety of valley configurations, in both weak and strong charge-noise regimes. When the charge noise is weak, high fidelity qubits can be implemented across a wide range of valley parameters, provided the electronic pulse is fine-tuned for a given valley configuration. When the charge noise is strong, high-fidelity pulses can still be engineered, provided the valley splittings in each dot are relatively large and the valley phase difference is relatively small. We analyze how charge noise-induced fluctuations of the inter-dot detuning, as well as small shifts in other qubit parameters, impact qubit fidelities. We find that strongly driven pulses are less sensitive to detuning fluctuations but more sensitive to small shifts in the valley parameters, which can actually dominate the qubit infidelities in some regimes. Finally, we discuss schemes to tune devices away from poor-performing configurations, enhancing the scalability of flopping-mode-based qubit architectures.
Itinerant antiferromagnetism in the antagonistic pair compound Y$_4$Co$_3$Ag
Low dimensional crystallographic motifs have long been associated with desirable physical properties. The confinement of electrons to low dimensions is thought to enhance quantum fluctuations and may promote correlated phenomena. Here, using the antagonistic pair concept, we add Y to the immiscible Co-Ag pair to discover Y$_4$Co$_3$Ag. This compound adopts a monoclinic $I$2/$m$ structure consisting of Y channels that are filled by one-dimensional zigzag and hexagonal Co chains, which extend along the crystallographic $b$-axis with no nearest neighbor contacts between Co and Ag atoms. Transport, magnetic, and specific heat measurements reveal that Y$_4$Co$_3$Ag orders antiferromagnetically at $T_N=14.9$ K with an effective magnetic moment $\mu_{\text{eff}}$ = 1.4 $\mu_{\text{B}}$/Co. Specific heat measurements show only a small entropy loss on the order of $0.1\,R\ln2$ associated with magnetic order, and magnetization isotherms, in DC fields up to 70 kOe at 1.8 K and in pulsed fields up to 600 kOe at 500 mK, indicate a small ordered moment of less than 0.2 $\mu_B$/Co. Taken together, our results imply the presence of small, itinerant moments and strong fluctuations in Y$_4$Co$_3$Ag, suggesting that Y$_4$Co$_3$Ag may be a promising candidate material to investigate itinerant magnetic interactions in a quasi-one dimensional system.
Charge-sensitive vibrational modes in BEDT-TTF salts: Signatures of charge ordering and site charge
BEDT-TTF-based organic conductors host a number of ground states, tuned by electron repulsion from Mott and charge ordered insulators to superconductors. Knowing charge distribution on the molecular sites in the insulating state of these materials is a key to understanding the origin of these ground states. We survey and discuss the C=C stretching modes in BEDT-TTF based molecular conductors. These molecular vibrations are extremely crucial in characterization of charge-ordered insulators, and are recently linked to superconductivity in some compounds. Focusing on the known examples of BEDT-TTF$^{+0.5}$ salts, we analyse the reliability of the C=C stretching modes for the determination of charge ordering and absolute site charge. Considering the charge-ordered states, a prominent shift in frequency of 141 cm$^{-1}$ per elementary charge $e$ for $\nu_{27}(b_{1u})$ and 98 cm$^{-1}$$e$ for $\nu_2$($a_g$) can be clearly realised, however, the distribution resulting from different compounds span over 20 cm$^{-1}$. For nominal BEDT-TTF$^{+0.5}$ compounds, the distribution of the resonance also extends around 20 cm$^{-1}$, yielding an unexpected large uncertainty of $\Delta\rho~\approx~(~\pm~0.045)e$, which is presumably due to the influence of small differences in the structure. This highlights the limitations of charge-frequency relations to detect small deviations in absolute charge values on molecular lattice sites, and emphasises on the use of the relations to estimate charge-ordering, rather than absolute site charge.
Beyond Commutativity: Redesigning Trotter Decomposition via Local Symmetry
The product formula, commonly known as Trotter decomposition, is a central tool for digital quantum simulation, whose performance depends critically on how the Hamiltonian is partitioned into tractable blocks. Standard decompositions typically rely on direct commutativity among Hamiltonian terms in a chosen operator representation, which can lead to large residual errors and deep circuits for complex, practically relevant many-body quantum systems. We address this fundamental bottleneck by introducing a new decomposition principle that goes beyond commutativity, grouping Hamiltonian terms into local three-site clusters according to the underlying SU(2) symmetry of the local dynamics. We show that three-site generators fall into at most four SU(2)-symmetry classes, each admitting an effective two-qubit SU(4) representation with exact and efficient implementations. By reducing the number of clusters, this decomposition principle substantially suppresses commutator-induced errors and circuit overhead while preserving underlying physical structures that commutativity-based decompositions may violate. We demonstrate the proposed method on several physically relevant spin-lattice models, where the reduced cluster structure can even realise the second-order product formula without doubling the circuit depth, as would be required by conventional decompositions. Numerical simulations of a Kagome Heisenberg model with triangular spin-chirality interactions show that the proposed method reduces both state infidelity and average spin-chirality bias by more than three orders of magnitude compared with conventional decompositions, while using substantially fewer gates. These results establish local symmetry as a flexible and practical design principle for product-formula simulation, opening a route to more accurate and hardware-efficient simulations of broader classes of many-body systems.
Born-rule statistical dynamical quantum phase transitions under measurement
Dynamical quantum phase transitions (DQPTs) occur at times when a quantum state exhibits a nonanalytic change in its return probability. This can be viewed as the probability of collapsing the evolved state to the initial state by quantum measurement. However, the initial wave function usually has exponentially small amplitude in the late time evolved state. Here we perform statistical characterization for all the possible post-measurement states distributed according to the Born's rule, by sampling a one-dimensional quantum Ising chain after a quantum quench dynamics. The statistical ensemble can also be viewed as a mixed state when the time evolved state is subjected to maximally dephasing noise in a certain basis. We map the distribution to a statistical model and characterize its effective "energy" spectrum, and introduce the average dynamical free energy, establishing a framework for the statistical DQPTs. We show the recovering of DQPT under high-moment average and a delocalized level distribution following critical times. Through analytic continuation into the complex time plane, we demonstrate the vanishing of Yang-Lee-Fisher zeros and the emergent level crossing near critical times. Finally, we propose a measurement-based quantum computation protocol to simulate the unitary evolution via single-qubit measurements on a two-dimensional cluster state. Our results provide a way for experimentally investigating statistical DQPTs in quantum devices, shedding light on the structured circuit sampling with insights from DQPT and generalizing the understanding of mixed state due to decoherence beyond equilibrium.
Deconfined quantum criticality with internal supersymmetry
Deconfined quantum critical point (DQCP) describes direct, non-fine-tuned quantum phase transition between two ordered phases that break distinct and seemingly unrelated symmetries, providing a route to continuous phase transition beyond the conventional Ginzburg--Landau paradigm. In this work we extend the DQCP paradigm to systems with internal supersymmetry (SUSY), where the on-site Hilbert space furnishes a representation of a Lie superalgebra, and the Hamiltonian is invariant under the corresponding Lie supergroup. Focusing on the minimal supersymmetric generalization of spin $SU(2)$, namely $OSp(1|2)$, we propose a supersymmetric deconfined quantum critical point (sDQCP) between a phase that breaks internal $OSp(1|2)$ and a phase that instead breaks lattice rotation symmetry. We formulate a non-linear sigma model on the supersphere target space that captures the symmetry intertwinement characteristic of the sDQCP, and we further develop a gauge theory description to address its dynamical properties, including a heuristic argument for 3D XY critical behavior. Finally, we show that explicitly breaking $OSp(1|2)$ down to $SU(2)$ continuously connects our sDQCP to the conventional DQCP scenario.
Local Topological Quantum Order and Spectral Gap Stability for the AKLT Models on the Hexagonal and Lieb Lattices
We prove that the ground state of the AKLT models on the hexagonal lattice and the Lieb lattice satisfy the local topological quantum order (LTQO) condition. This will be a consequence of proving that the finite volume ground states are indistinguishable from a unique infinite volume ground state. Concretely, we identify a sequence of increasing and absorbing finite volumes for which any finite volume ground state expectation is well approximated by the infinite volume state with error decaying at a uniform exponential rate in the distance between the support of the observable and boundary of the finite volume. As a corollary to the LTQO property, we obtain that the spectral gap above the ground state in these models is stable under general small perturbations of sufficient decay. We prove these results by a detailed analysis of the polymer representation of the ground states state derived by Kennedy, Lieb and Tasaki (1988) with the necessary modifications required for proving the strong form of ground state indistinguishability needed for LTQO.
Chemical Origins of Non-Bonded Interactions Within and Between Solids
Non-bonded interactions govern structure, stability, and function across a wide range of solid-state materials, yet their chemical origins are often difficult to resolve from total energies alone. Here we generalize absolutely localized molecular orbital energy decomposition analysis to quantify and interpret non-bonded interactions within and between solids at the density functional theory level. Across molecular crystals, moir\'e heterobilayers, and layered perovskite heterostructures, this framework separates lattice-formation energies, interlayer binding energies, and band-structure changes into chemically intuitive contributions from frozen interactions, polarization, and charge transfer. The analysis reveals how dispersion controls polymorph stability in pharmaceutical crystals, how local stacking modulates interlayer coupling in MoS2/WSe2, and how alkali-cation substitution switches the quantum-well character of layered perovskite heterostructures. By connecting emergent solid-state properties to microscopic interaction mechanisms, this framework provides a chemically transparent basis for understanding and designing complex materials.
Interfacial Reconstructions and Engineering in III-V@II-VI Core-Shell Quantum Dots
In core/shell quantum dots (QDs), the interface between semiconductors of different chemical character largely determines their optoelectronic properties. In III-V/II-VI systems, this boundary involves pronounced chemical and electronic discontinuities that can generate trap states even under complete surface passivation. Using density functional theory on atomistic models of InAs/CdSe QDs, we systematically reconstruct atomic arrangements at the surface and interface to evaluate how local coordination and interfacial dipoles influence the electronic structure. Abrupt interfaces induce charge imbalance and band-gap collapse, whereas introducing an alloyed interlayer that mixes core and shell atoms and vacancies restores energetic alignment and yields delocalized band-edge states, consistent with experimental findings. We also introduce a charge-flow analysis that quantifies charge redistribution across the QD, providing a framework for realistic modeling of interlayer formation and predictive design of defect-free interfaces in core@shell architectures.
Charge Transfer from Perovskite Quantum Dots to Multifunctional Ligands with Tethered Molecular Species
That author's affiliation: Ludwig-Maximilians-Universität München Institution (first & last author): Ludwig-Maximilians-Universität München
Perovskite quantum dots (pQDs) are promising materials for optoelectronic and photocatalytic applications due to their unique optical properties. To enhance charge carrier extraction or injection donor/acceptor molecules can be tethered to the pQD. These molecules must strongly bind to the ionic surfaces of pQDs without compromising colloidal stability. These we achieve by using multifunctional ligands containing a quaternary ammonium binding group for strong pQDs surface attachment, a long tail group for colloidal stability, and a functional group near the pQD surface. Such pQDs with ferrocene-functionalized ligands show fast photoexcited hole transfer with near-unity efficiency. Density functional theory calculations reveal how ferrocene's molecular structure reorganizes following hole transfer, affecting its charge separation efficiency. This approach can also be extended to in photoexcited electron and energy transfer processes with pQDs. Therefore, this strategy offers a blueprint for creating efficient QD-molecular hybrids for applications like photocatalysis.
Non-Relativistic Spin-Orbit Interaction in Triplet Superconductors: Edelstein Effect and Spin Pumping by Electric Fields
Non-relativistic momentum-dependent spin splitting, as observed in collinear altermagnets and non-collinear $p$-wave magnets, provides exciting avenues for controlling spin dynamics. Here, we reveal a distinct form of non-relativistic ``spin-orbit coupling" in triplet superconductors by demonstrating that the triplet order parameter induces a wave-vector-dependent spin texture of Bogoliubov quasiparticles, thereby entangling their orbital and spin motions. Even in the absence of relativistic spin-orbit coupling, this intertwining of spin and orbital motion allows an electric field to generate spin polarization in a $p$-wave superconductor -- that is, an Edelstein effect. Building on this mechanism, we propose an efficient scheme for the nonlinear generation of a DC spin current via electric near fields, driven by AC spin polarization and electron velocity. This general principle offers a powerful route for generating and manipulating spin currents in unconventional superconductors.
Inherent momentum-dependent gap structure of altermagnetic superconductors
Altermagnetic metals break time-reversal symmetry and feature spin-split Fermi surfaces generated by compensated N\'eel-ordered collinear magnetic moments. Being metallic, such altermagnets may undergo a further instability at low temperatures to a superconducting state, and it is an interesting open question what the salient features are of such altermagnetic superconductors. We address this question on the basis of realistic microscopic models that capture the altermagnetic sublattice degrees of freedom. We find that the sublattice structure can strongly affect the superconducting gap structure in altermagnetic superconductors. In particular, it imposes nodes in the gap on the Brillouin zone edges for superconductors stabilized by momentum-independent bare attraction channels. We contrast this to the case of superconductivity generated by extended range interactions where pairing is allowed on the Brillouin zone edges and both spin-singlet and equal-spin-pairing triplet states can be stabilized. Equal-spin-pairing triplet superconductivity is generically favored in the limit of large altermagnetic spin splitting of the bands compared to the superconducting gap scale, and features characteristic nonunitary properties arising from the altermagnetic order.
Reentrant Superconductivity from Competing Spin-Triplet Instabilities
Reentrant superconductivity in strong magnetic fields challenges the conventional expectation that magnetic fields necessarily suppress superconductivity. We show that reentrant superconducting instability can arise from the competition between spin-unpolarized and spin-polarized superconducting channels. Using a minimal Ginzburg--Landau theory with two coupled spin-triplet order parameters, we demonstrate that a magnetic field can reorganize the hierarchy of superconducting instabilities, yielding a characteristic reentrant instability curve over a broad parameter range.
Generalized Toffoli gates with customizable single-step multiple-qubit control
That author's affiliation: National Taiwan University Institution (first & last author): National Taiwan University
Generalized Toffoli gates with customizable single-step multiple-qubit control
Bounding the computational power of bosonic systems
Bounding the computational power of bosonic systems
Controllable hydro-thermoelastic heat transport in ultrathin semiconductors at room temperature
That author's affiliation: Institut Català de Nanociència i Nanotecnologia First author institution: Eindhoven University of Technology Last author institution: Institut Català de Nanociència i Nanotecnologia
The combination of viscous heat flow and thermoelastic effects leads to a non-diffusive heat transport regime in MoSe2 and MoS2. Moreover, it can be controlled through the variation in sample thickness and by choosing between continuous and pulsed heating.
Spatially anisotropic Kondo resonance coupled with the superconducting gap in a kagome metal
How magnetic impurities influence superconductivity and electronic order in kagome metals remains unclear. Now anisotropic Kondo resonances intertwined with the superconducting gap are observed in a magnetically doped kagome superconductor.
Cryogenic microwave frequency combs based on quantum paraelectric superconducting resonators
A frequency comb, known for its precision as an "optical ruler", features an evenly spaced spectral pattern. While these combs are vital in photonic quantum technologies, their microwave counterparts are now highly sought after for cryogenic quantum technologies, including semiconducting and superconducting qubits and quantum electrical metrology, which mainly operate in the microwave regime. However, microwave combs are still largely underexplored, and typically rely on complex, high-power optical systems incompatible with the low-power, cryogenic on-chip quantum technologies. In this manuscript, we present an all-electrical, on-chip, cryogenic microwave frequency comb on Strontium Titanate (SrTiO$_3$), exploiting its Pockels-like effect in its quantum paraelectric phase. Our device, utilizing a superconducting microwave cavity, generating the frequency comb via cavity phase modulation enabled by the field-induced effective $\chi(2)$ of SrTiO$_3$. The ability to continuously vary the dielectric constant of SrTiO$_3$ by the application of electric field, in its quantum paraelectric phase, makes it possible to control the comb's operating frequency range. The exceptionally high dielectric constant of SrTiO$_3$, > 20,000 in its quantum paraelectric state, enables an ultra-miniature design and on-chip integration with cryogenic quantum technologies.
Shubnikov-de Haas Characterization of Superconductor-Semiconductor Heterostructures
Hybrid superconductor-semiconductor nanostructures are a central component for research spanning condensed matter physics and quantum information processing. Continued progress relies critically on the ability to characterize, control, and optimize several intrinsic material properties including spin-orbit coupling, band offsets, and disorder in a device-relevant stack that necessarily couples the electronic states of a superconducting metal film and a semiconductor. Here we report a new method to extract fundamental material parameters utilizing simple Shubnikov-de Haas (SdH) oscillation measurements in heterostructures in which metallic electronic states are coupled to a two-dimensional electron gas (2DEG) residing in an InAs quantum well beneath an aluminum thin film. Proper analysis of the full magnetoresistance data facilitates extraction of the quantum well carrier density, spin-orbit coupling strength, and both transport and quantum scattering times. Most importantly, the extracted scattering times in the 2DEG are impacted by the metal-semiconductor coupling strength allowing us to quickly gain information on proximity-induced superconducting gap without any fabrication or mK measurements. The wealth of information that is accessed with these simple measurements positions this methodology as an important tool for hybrid materials optimization.
Interface controlled spin filtering and nonreciprocal transport in Altermagnet/Ising superconductor junctions
We investigate theoretically spin-resolved transport, spin filtering, and nonreciprocal effects in an Altermagnet/Ising superconductor (AM/ISC) junction with a spin-active interface. Using a modified Bogoliubov-de Gennes framework within the scattering formalism, we demonstrate that the interplay among intrinsic spin-orbit coupling (ISOC), anisotropic AM spin texture and spin-dependent interfacial scattering gives rise to strongly anisotropic charge and spin conductance. In the weak spin-mixing regime, transport remains predominantly helicity conserving and exhibits pronounced angular dependence governed by the relative orientation between the AM spin texture and interface magnetization. Increasing ISOC enhances spin conductance and leads to spin-selective Andreev reflection resulting in finite spin filtering. In contrast, the strong spin-mixing regime exhibits enhanced angular anisotropy and robust spin-polarized transport over a broad energy range. Conventional Andreev reflection becomes strongly suppressed, accompanied by substantial spectral redistribution. We further show that nonreciprocal transport persists throughout the single-band, intermediate and double-band ISC regime. The spin polarization and spin-filter efficiency exhibit nonmonotonic dependence on system parameters, reaching values up to $\sim 86\%$, with characteristic angular modulation determined by the AM spin texture. Finite-energy analysis reveals enhanced spin selectivity at low energies and suppression near the superconducting gap. Furthermore, strong spin mixing at the AM/ISC junction produces asymmetric conductance patterns, indicating nonreciprocal transport. Our results establish AM/ISC junctions as a versatile platform for tunable superconducting spintronics and directional spin transport.
Negative Spin $\Delta_T$ noise Induced by Spin-Flip Scattering and Andreev Reflection
We study charge $\Delta_T$ noise, followed by an examination of spin $\Delta_T$ noise, in the normal metal-spin flipper-normal metal-insulator-superconductor (N-sf-N-I-S) junction. Our analysis reveals a key contrast: while charge $\Delta_T$ noise remains strictly positive, spin $\Delta_T$ noise undergoes a sign reversal from positive to negative, driven by the interplay between spin-flip scattering as well as Andreev reflection. In contrast, charge quantum shot noise remains positive and sign-definite, which is also valid for spin quantum shot noise. The emergence of negative spin $\Delta_T$ noise has two major implications. First, it establishes a clear distinction between spin-resolved $\Delta_T$ noise and quantum shot noise: the former is dominated by opposite-spin correlations, whereas the latter is led by same-spin correlations. Second, it provides access to scattering mechanisms that are not captured by quantum shot noise alone. Thus, negative spin $\Delta_T$ noise serves as a unique probe of the cooperative effects of Andreev reflection and spin flipping. We further place our results in context by comparing them with earlier reports of negative $\Delta_T$ noise in strongly correlated systems, such as fractional quantum Hall states, and in multiterminal hybrid superconducting junctions. Overall, this work offers new insights into the mechanisms governing sign reversals in $\Delta_T$ noise and highlights their role as distinctive fingerprints of spin-dependent scattering in superconducting hybrid devices.
Vestigial Gapless Boson Density Wave Emerging between $\nu = 1/2$ Fractional Chern Insulator and Finite-Momentum Supersolid
The roton-triggered charge-density-wave (CDW)is widely studied in fractional quantum Hall (FQH) and fractional Chern insulator (FCI) systems, and there also exist field theoretical and numerical realizations of continuous transition from FCI to superfluid (SF). However, the theory and numerical explorations of the transition between FCI and supersolid (SS) are still lacking. In this work, we study the topological flat-band lattice models with $\nu$ = 1/2 hard-core bosons, where the previous studies have discovered the existence of FCI states and possible direct FCI-SS transitions. While the FCI is robust, we find the direct FCI-SS transition is absent, and there exist more intriguing scenarios. In the case of checkerboard lattice, we find an intermediate gapless CDW state without SF, sandwiched between FCI and SS. This novel state is triggered by the roton instability in FCI and it further continuously brings about the intertwined finite-momentum SF fluctuation when the CDW order is strong enough, eventually transiting into an unconventional finite-momentum SS state. The intermediate gapless CDW state is a vestige from the SS state, since the increasing quantum fluctuation melts only the Larkin-Ovchinnikov-type SF order in SS but its (secondary) product -- the CDW order -- survives. On honeycomb lattice, we find no evidence of SS, but discover an interesting sequence of FCI-Solid I-Solid II transitions, with both solids incompressible. Moreover, in contrast to previous single-roton condensation, this sequence of FCI-Solid I-Solid II transitions is triggered by the softening of multi-roton modes in FCI. Considering the intertwined wave vectors of the CDW orders, Solid I is a vestige of Solid II. Our work provides new horizon not only for the quantum phase transitions in FCI but also for the intertwined orders and gapless states in bosonic systems, which will inspire future studies.
Slave-spin approach to the Anderson-Josephson quantum dot
That author's affiliation: Institut de Physique Institution (first & last author): Institut de Physique
We study a strongly interacting quantum dot connected to two superconducting leads using a slave-spin representation of the dot. At the mean-field level, the problem maps to a resonant level model with superconducting leads, coupled to an auxiliary spin-1/2 variable accounting for the parity of the dot. We obtain the mean-field phase diagram, showing a transition between a Kondo (singlet) and a local moment (doublet) regime, corresponding to the $0-\pi$ transition of the junction. The mean-field theory qualitatively captures the Kondo singlet phase and its competition with superconductivity for weak values of the BCS gap, including the non-trivial dependence of the Andreev bound states on the interaction, but fails in the doublet regime where it predicts a dot decoupled from the bath. Using diagrammatic techniques and a random phase approximation, we include fluctuations on top of the mean-field theory to describe finite-frequency dynamics of the effective spin variable. This leads to the formation of high-energy Hubbard bands in the spectral function and a coherent Kondo peak with a BCS gap at low energies. We compute the Josephson current and the induced superconducting correlations on the dot. Finally, we evaluate the microwave response in the strongly interacting Kondo regime.
Ballistic-to-diffusive transition in engineered counter-propagating quantum Hall channels
Exotic quantum Hall systems hosting counter-propagating edge states can show seemingly non-universal transport regimes, usually depending on the size of the sample. We experimentally probe transport in a quantum Hall sample engineered to host a tunable number of counter-propagating edge states. The latter are coupled by Landauer reservoirs, which force charge equilibration over a tunable effective length. We show that charge transport is determined by the balance of up- and downstream channels, with a ballistic regime emerging for unequal numbers of channels. For equal numbers, we observe a transition to a critical diffusive regime, characterized by a diverging equilibration length. Our approach allows simulating the equilibration of hole-conjugate states and other exotic quantum Hall effects with fully controlled parameters using well-understood quantum Hall states.
Quantum-Limited Acoustoelectric Amplification in a Piezoelectric-2DEG Heterostructure
We provide a quantum mechanical description of phonon amplification in a heterostructure consisting of a two-dimensional electron gas (2DEG) stacked on top of a piezoelectric material. An applied drift voltage effectively creates a population inversion in the momentum states of the 2DEG electrons, giving rise to spontaneous emission of phonons. Once an acoustic wave is launched, the pumped electrons release phonons via stimulated emission, returning to depleted ground states before being pumped back to the excited states. We show that whereas efficient amplification using a 1D electron gas requires the acoustic wavelength to roughly equal the average electron-electron spacing, a 2DEG enables efficient amplification for any wavelength greater than the average electron-electron spacing. We derive the imaginary and real parts of the 2DEG first-order acoustic susceptibility as functions of electronic drift velocity in specific limits and derive the gain per unit length for the signal and the quantum noise, with the gain matching the classical result in the short-electronic-lifetime (low-mobility) regime. Moreover, we analyze the gain clamping due to pump depletion and calculate the maximum achievable intensity. Our results provide a framework for designing novel acoustic devices including a quantum phononic laser and phase-insensitive quantum phononic amplifiers.
Correlated Quantum Phenomena in Confined Two-Dimensional Hexagonal Crystals
Low-energy fermionic excitations in two-dimensional materials deviate from the conventional Schr\"odinger description and are instead governed by Dirac equations. Such Dirac fermions give rise to a variety of unconventional quantum phenomena that have no direct analogues in traditional condensed matter systems. Among these materials, graphene and transition metal dichalcogenides (TMDs) represent two prototypical platforms, hosting massless and massive Dirac particles, respectively, and exhibiting rich electronic, optical, and valley dependent properties. Here we review the effect of the quantum confinement in these two-dimensional hexagonal materials that provides a powerful route to enhance Coulomb interactions and stabilizing correlated quantum states. In graphene- and TMD-based quantum dots, externally imposed confinement leads to discrete electronic and excitonic spectra, where interaction effects are strongly amplified. In twisted van der Waals heterostructures, the moir\'e superlattices generate emergent confinement and induce nontrivial band topology, giving rise to a wealth of novel phenomena. More generally, reduced dimensionality and spatial localization in two-dimensional materials promote a diverse range of correlated states. Recent experimental and theoretical advances highlight the central role of confinement in shaping quantum behavior and reveal new opportunities for applications based on these states. In this review, we provide an overview of recent progress in confinement-induced correlated phenomena in two-dimensional materials from both theoretical and experimental perspectives.
Universal quantum melting of quasiperiodic attractors in driven-dissipative cavities
That author's affiliation: Universität Hamburg First author institution: Universität Hamburg Last author institution: University of Konstanz
Nonlinear classical mechanics has established rich phenomena. These include limit tori defined by toroidal attractors supporting quasiperiodic motion with incommensurate frequencies. We study the fate of such structures in open quantum systems using two coupled driven-dissipative Kerr cavities modeled via the Lindblad master equation. Combining Liouvillian spectral theory with the truncated Wigner approximation, we characterize the quantum-to-classical crossover. In the classical limit, two pairs of purely imaginary Liouvillian eigenvalues signal persistent quasiperiodic modes. Quantum fluctuations induce small negative real parts to these eigenvalues, giving rise to finite lifetimes and leading to the quantum melting of the torus. The associated Liouvillian gaps vanish algebraically in the classical limit, indicating a dynamical critical crossover with spontaneous breaking of time-translational symmetry. Quantum trajectory analysis reveals that this melting is driven by fluctuation-induced dephasing. Using a circular-variance-based order parameter, we uncover universal scaling in system size and time. These results establish quantum melting of limit tori as a distinct and robust non-equilibrium critical phenomenon, with clear experimental signatures in trapped ions and superconducting circuits.
Scalable Spin Qubit Architecture with Donor-Cluster Arrays in Silicon
Spin qubits in silicon donors offer a promising platform for quantum computing due to their long coherence times and semiconductor compatibility. However, scaling donor-based spin qubits in silicon is fundamentally challenged by frequency crowding, crosstalk, and the tight tolerances on donor placement in conventional single-donor architectures.To overcome this, we introduce a paradigm based on a two-dimensional array of phosphorus-donor clusters, in which multiple donors share a bound electron. The natural hyperfine distribution within each cluster enables individual addressability of the electron and nuclear spins, while tunable exchange interactions between clusters mediate local all-to-all connectivity. We present a universal control protocol achieving gate fidelities exceeding 99% for both intra-cluster and inter-cluster multi-qubit operations, with crosstalk effectively suppressed. The architecture natively supports efficient quantum error correction, including bias-tailored codes that exploit the intrinsic noise bias of spin qubits. Furthermore, its modular design is compatible with long-range coupling via electron shuttling for large-scale integration. This donor-cluster array architecture establishes a robust and hardware-efficient pathway towards scalable, fault-tolerant quantum computing in silicon.
Imaging Interacting Two-Dimensional Anisotropic Electrons
We directly visualize a two-dimensional anisotropic Wigner crystal and its quantum melting in monolayer 1T-ReSe2 using non-invasive scanning tunnelling microscopy. In crystals with anisotropic effective mass, an electron's quantum wavefunction becomes elongated along the light-mass direction to reduce kinetic energy. At low electron density, such anisotropic electrons are predicted to form an oblique Wigner crystal rather than the familiar triangular lattice of isotropic systems. Despite longstanding theoretical interest, this physics has been little explored experimentally. Here we first image the anisotropic shape of individual electrons in gated monolayer ReSe2, whose wavefunctions are strongly elongated along the light-mass direction. At low density, these electrons crystallize into an oblique Wigner lattice. As the density increases, quantum fluctuations grow more rapidly along the light-mass direction than along the heavy-mass direction, driving a one-dimensional melting of the crystal. The resulting state retains order along one direction but melts along the other, consistent with a smectic electron liquid crystal between the electron solid and Fermi liquid phases. Our work establishes monolayer ReSe2 as a platform for studying anisotropic correlated electrons, quantum melting, and coupled one-dimensional electron chains.
Parallel Scan Recurrent Neural Quantum States for Scalable Variational Monte Carlo
Neural-network quantum states have emerged as a powerful variational framework for quantum many-body systems, with recent progress often driven by massively parallel architectures such as transformers. Recurrent neural network quantum states, however, are frequently regarded as intrinsically sequential and therefore less scalable. Here we revisit this view by showing that modern recurrent architectures can support fast, accurate, and computationally accessible neural quantum state simulations. Using autoregressive recurrent wave functions together with recent advances in parallelizable recurrence, we develop variational ans\"atze, called parallel scan recurrent neural quantum states (PSR-NQS), which can be trained efficiently within variational Monte Carlo in one and two spatial dimensions. We demonstrate accurate benchmark results and show that, with iterative retraining, our approach reaches two-dimensional spin lattices as large as $52\times52$ while remaining in agreement with available quantum Monte Carlo data. Our results establish recurrent architectures as a practical and promising route toward scalable neural quantum state simulations with modest computational resources.
Quantum geometric ferromagnetism by singular saddle point
We propose ferromagnetism that occurs in electrons at a saddle point with band touching, which we call the singular saddle point. At the singular saddle point, the divergent quantum metric induces ferromagnetic correlation, and the logarithmic divergence of the density of states ensures ferromagnetism within Stoner theory. This is a prototypical example of quantum geometric ferromagnetism. The two-dimensional $t_{2g}$-orbital model accommodates the ferromagnetism by this mechanism, which is continuously connected to the exactly proven flat-band ferromagnetism.
Collective excitations in chiral spin liquid: chiral roton and long-wavelength nematic mode
Chiral spin liquid (CSL) is a magnetic analogue of the fractional quantum Hall (FQH) liquid. Collective excitations play a vital role in shaping our understanding of these exotic quantum phases of matter and their quantum phase transitions. While the magneto-roton and long-wavelength chiral graviton modes in the FQH liquids have been extensively explored, the collective excitations of CSLs remain elusive. Here we explore the collective excitations in the SU(2) symmetric CSL phase of the spin-1/2 square-lattice $J_1-J_2-J_\chi$ model, where an intriguing quantum phase diagram was recently revealed. Combining exact diagonalization and time-dependent variational principle calculations, we observe two spin-singlet collective modes: a chiral p-wave (low-energy) roton mode at finite momentum and a elliptically polarized d-wave (higher-energy) nematic mode at zero momentum, both of which are prominent across the CSL phase. Such exotic modes exhibit fingerprints distinct from those of FQH liquids, and to the best of our knowledge, are reported for the first time. By tuning $J_2$, we find the nematic mode to be pronouncedly soft, together with the spin-triplet two-spinon bound states, potentially promoting strong nematic and spin stripe instabilities. Our work paves the way for further understanding CSL from the dynamical perspective and provides new spectroscopic signatures for future experiments of CSL candidates.
Chirality-Induced Spin Selectivity: Nonlinear Spin Response from Electron-Phonon Scattering
Chirality-induced spin selectivity (CISS) generates spin-polarized currents in nonmagnetic materials from structural chirality alone, yet its microscopic origin remains debated. Using a first-principles spatiotemporal density-matrix dynamics approach including electron-phonon scatterings with self-consistent spin-orbit coupling (SOC), we elucidate the interplay of SOC, structural chirality, and spin-dependent electron-phonon interactions in driving the generation and transport of spin and orbital angular momentum. In particular we quantitatively distinguish CISS from the collinear Edelstein effect (CEE) in trigonal selenium, a prototypical chiral solid. CEE yields a spatially uniform spin polarization scaling linearly with applied field ($S_z \propto E$). In contrast, explicit spin-dependent electron-phonon scattering produces a nonlinear response ($S_z \propto E^2$) and a length-dependent spin accumulation -- the hallmark experimental signature of CISS. We identify intervalley scattering mediated by chiral phonon angular momentum as the microscopic origin of this nonlinearity.
Understanding oxide-thickness-dependent variability in dense Si-MOS quantum dot arrays
Achieving uniform and scalable control of semiconductor spin qubits remains a key challenge for large scale quantum computing. In this work, we investigate how gate oxide thickness influences uniformity in dense two dimensional silicon quantum dot arrays. Using a 7 x 7 array fabricated in a 300 mm CMOS-process patterned by EUV lithography, we statistically characterize 392 quantum dots across four different oxide thicknesses. The threshold voltages, capacitances, lever arms, and charging energies are extracted using parallel row based measurements and we identify an optimal SiO2 thickness of 17 nm that minimizes threshold voltage variability below 63 mV standard deviation. Our observations illustrate how multiple sources of disorder can introduce competing oxide-thickness dependencies, resulting in non-monotonic trends. These results provide key design guidelines for dense, scalable silicon spin qubit architectures.
Quantum computational sensing using quantum signal processing, quantum neural networks, and Hamiltonian engineering
Quantum computational sensing using quantum signal processing, quantum neural networks, and Hamiltonian engineering
Practical blueprint for low-depth photonic quantum computing with quantum dots
Practical blueprint for low-depth photonic quantum computing with quantum dots
Rashba engineering at van der Waals interfaces
Two-dimensional transition metal dichalcogenide (TMD) interfaces offer a versatile platform for studying emergent quantum phenomena and enabling novel device functionalities. When distinct TMD monolayers are stacked vertically or laterally stitched, their interfaces can exhibit unique electronic band alignments, giving rise to long-lived interlayer excitons, charge transfer effects, and moir\'e superlattices with correlated states. Here, we demonstrate that the interface between a large variety of two different epitaxially grown TMD monolayers controls the intensity and sign of the Rashba spin splitting, which is probed using THz spintronic emission. Optimized TMD heterobilayers, such as HfSe$_2$/PtSe$_2$, show enhanced THz emission that surpass the spin-to-charge conversion efficiency of bulk TMDs, confirming the presence of Rashba states with large spin splitting at the interface. By combining spin- and angle-resolved photoemission spectroscopy with density functional theory, we reveal that the electronic hybridization between the two different TMD monolayers gives rise to extended in-gap states with strong Rashba spin-orbit coupling. The choice of TMD layers enables to engineer the sign and strength of spin-to-charge conversion in van der Waals heterobilayers opening up perspectives to build efficient and tunable THz spintronic emitters.
Emergent Quantum-Geometric Equivalence of Injection and Shift Currents
Injection and shift currents are generally regarded as distinct nonlinear optical responses with separate microscopic origins. Here, we uncover a general hidden connection between them through interband Berry-curvature and quantum-metric dipoles. In systems with approximately linear electronic dispersion near the Fermi level and at low photon energies, this relation sharpens into an emergent equivalence, with injection and shift currents governed by the same interband quantum-geometric dipole. This regime is naturally realized in Dirac and Weyl semimetals, as well as in strained graphene, where measurements of injection and shift currents probe a unified geometric property of the electronic wavefunctions rather than distinct dynamical processes. Our results establish a new framework for interpreting nonlinear optical experiments and suggest that quantum geometry may provide a broader organizing principle linking seemingly distinct nonlinear optical responses in solids.
Coherence, long-range transport and nuclear polarization in a driven-dissipative dark exciton condensate
We report direct evidence for macroscopic coherence in a condensate of dark dipolar excitons in coupled quantum wells and show that its formation follows a non-equilibrium, driven-dissipative mechanism. The condensation transition is governed by gain-loss competition, in which the exceptionally long lifetime of dark excitons enables their dominance in mode selection. Condensate formation is revealed by photoluminescence darkening, changes in radiative recombination channels, and the emergence of long-range hydrodynamic transport manifested by propagation of density (sound) modes over millimeter-scale distances. The buildup of dark exciton density induces dynamic nuclear polarization, which closes the dark-bright exciton gap, \Delta, via the Overhauser field. This leads to nuclear spin polarization across the entire mesa, far beyond the optically excited region, and produces pronounced hysteresis behavior. At \Delta ~ 0 the gap is locked and the condensate loss are minimal, resulting in a second threshold manifested as a photoluminescence blueshift. Coherence is revealed through interference between incident and boundary-reflected exciton currents, producing spatial modulation of the photoluminescence from the radiative reservoir and enabling extraction of the condensate coherence length. These results establish dark excitons as a platform for coherent quantum fluids in a driven-dissipative, strongly interacting regime with electrical tunability, bridging the physics of polariton condensates and matter-like excitonic systems.
Orbital and Spin Nernst Effects in Monolayers of Transition Metal Dichalcogenides
In recent years, orbitronic effects have attracted growing attention as complementary counterparts to the well-established spintronic phenomena. In this work, we demonstrate that monolayers of transition metal dichalcogenides provide an excellent platform for the observation of the orbital Nernst effect, a relatively less explored phenomenon describing the generation of a transverse orbital current in response to an applied temperature gradient. We show that, similar to its electrical counterpart, viz., the orbital Hall effect, the orbital Nernst effect does not require the presence of spin-orbit coupling. Analytical results based on a low-energy valley model offer key insights into the underlying mechanisms, highlighting in particular the crucial role of electronic states at the Fermi energy for the emergence of this effect. The inclusion of spin-orbit coupling further gives rise to a spin Nernst effect, which scales with the strength of spin-orbit coupling and vanishes in its absence. We substantiate our analytical findings with full Brillouin-zone tight-binding results for two representative systems, monolayer 2H MoS$_2$ and 2H NbS$_2$. Our results show that while both orbital and spin Nernst conductivities in MoS$_2$ require electron or hole doping, both effects are intrinsically present in metallic NbS$_2$. Our work reveals the central role of orbital and spin Berry curvatures, identifies doping as an effective route for tuning orbital and spin Nernst responses, and proposes a possible experimental setup for detecting these effects in monolayer transition metal dichalcogenides.
Cascade of fractional quantum Hall states in 2D system
That author's affiliation: Westlake University Institution (first & last author): Peking University
The observation of the fractional quantum Hall (FQH) effect in 2D electron gases ushered in investigations of topological phases driven by strong electron correlations. Their remarkable features include fractionalized elementary excitations, gapless boundary states, and non-trivial quantum entanglement patterns. Thanks to persistent efforts in the building of new platforms and making higher-quality samples, a diverse plethora of FQH states have been unveiled in experiments. We report a systematic study of ultrahigh-quality GaAs/AlGaAs quantum wells with mobility up to 3.7*10^7 cm^2/V/s using quantum transport measurements in nuclear adiabatic demagnetization and dilution refrigerators down to 1 mK. In addition to many FQH states that have already been identified in previous work, new longitudinal resistance dips are observed at filling factors 17/33 and 15/31. The application of an in-plane magnetic field causes disparate variations of the FQH states. The theoretical foundation of these states is discussed in the framework of composite fermion theory. While most fractions can be explained as non-interacting composite fermions forming integer quantum Hall states, a few states correspond to FQH states of composite fermions that arise from residual interaction between them. We summarize the observed fractions in the range of 0 < {\nu} < 2 and propose a pattern to account for their experimental appearance that provides an intuitive picture about the relative strengths of different FQH states.
Valley-contrasting Spin Textures in Janus Metal Phosphochalcogenides
Momentum-resolved spin textures and potential valley-contrasting physical properties in the momentum space are two intriguing characteristics of noncentrosymmetric materials, and they have broad applications in spintronics and valleytronics. The realization of diverse spin textures within a single material, along with their further coupling to the valley degree of freedom, is highly desirable. Via first-principles calculations, we investigate electronic properties of Janus MP$_2$S$_3$Se$_3$ monolayers, which exhibits distinct spin textures at different valleys. While Ising-type spin textures are located at $K_\pm$ valleys, the symmetry breaking from the Janus structure brings about a coexistence of Weyl-type and Rashba-type spin textures at $\Gamma$ valley. In addition to valley-contrasting spin textures, valley dependence also occurs in Berry-curvature-driven anomalous Hall currents and optical selectivity. Besides, energy differences between $\Gamma$ and $K_\pm$, as well as band gaps, are highly tunable by applied strain. These findings present an intriguing coupling between diverse spin textures and multiple valleys, and pave the way for designing advanced electronic devices that leverage spin and valley degrees of freedom.
Perspective on tailoring quantum coherence with electron beams
Examining and controlling the interaction between semiconductor quantum qubits and their environment can boost semiconductor quantum technologies, which have many applications in table-top quantum computing hardware. Electron beams in electron microscopes have opened up a new avenue for the quantum-coherent probing of semiconductor excitations and strong-coupling effects. Here, I provide a brief overview of recent advancements in electron-beam probes for investigating quantum coherence in semiconductors and two-dimensional materials, complemented by my perspective on using electron beams to manipulate the entanglement and correlations between quantum systems.
Ginzburg--Landau Theory for Confined Thin-Film Superconductors
We develop a Ginzburg--Landau theory for superconducting thin films under quantum confinement. Starting from the microscopic BCS free energy and the recently developed confinement theory of metallic thin films, explicit analytical expressions are derived for the Ginzburg--Landau coefficients, coherence length, penetration depth, electronic mean free path, and Ginzburg--Landau parameter in confined geometries. The central result is that quantum confinement directly renormalizes the intrinsic superconducting coherence length through confinement-induced modifications of the electronic density of states and Fermi energy. This effect is absent in conventional thin-film transport theories based solely on surface scattering. As a consequence, confinement simultaneously suppresses the coherence length and enhances the penetration depth, thereby driving superconductors toward progressively stronger type-II behavior with decreasing film thickness. The theory predicts a crossover regime in which confinement-induced renormalization of superconducting length scales and transport scattering become strongly intertwined. Comparison with recent penetration-depth measurements in Al thin films shows that the observed enhancement of the penetration depth originates from the interplay between confinement-induced renormalization of the coherence length and suppression of the effective mean free path by surface and disorder scattering. The results establish a direct connection between quantum confinement and superconducting electrodynamics in confined metallic films.
Super Moir\'e Domain Tessellations, Sliding Ferroelectricity, and Reconfigurable Quantum Dot Arrays in Twisted Trilayer Hexagonal Boron Nitride
At very small twist angles, bilayer moir\'e systems exhibit characteristic stacking domain patterns, where the moir\'e length scale is determined solely by the twist angle. In contrast, the additional stacking and twisting degrees of freedom in twisted trilayer systems give rise to richer and more intricate domain tessellations. In twisted trilayer hexagonal boron nitride (TTBN), the interplay between polar and nonpolar domains and their domain walls is shown to result in unconventional responses to external electric fields, including electric-field tunability of the moir\'e-of-moir\'e or super moir\'e pattern--features absent in bilayer counterparts. We demonstrate that at the vertices of super moir\'e domains, TTBN can support arrays of quantum dots hosting localized quantum harmonic oscillator (QHO) states with diverse spatial symmetries. Futhermore, we show that the shape of the array and the spacing between the localized QHO states can be dynamically reconfigured by electric fields, enabling facile switching between fully isolated and strongly coupled regimes. The local potentials for the quantum dot state are predicted to be sufficiently deep to support a series of QHO states with nonzero angular momentum. This tunability enables control over the transport of quantum dot states and their interdot coupling, facillitating long-range quantum state transfer. Combined with the feasibility of large-scale fabrication of homogeneous twisted trilayer materials, these properties position TTBN as a promising platform for a wide range of quantum technologies.
Holonomic quantum computation on graphene from Atiyah-Singer index theorem
We investigate the emergence of geometric phases in graphene-based nanostructures through the lens of the Atiyah-Singer index theorem. By modeling low-energy quasiparticles in curved graphene geometries as Dirac fermions, we demonstrate that topological defects arising from the insertion of pentagonal or heptagonal carbon rings generate effective gauge fields that induce quantized Berry phases. We derive a compact expression for the geometric phase in terms of the genus and number of open boundaries of the structure, providing a topological classification of zero-energy modes. This framework enables a deeper understanding of quantum holonomies in graphene and their potential application in holonomic quantum computation. Our approach bridges discrete lattice models with continuum index theory, yielding insights that are both physically intuitive and experimentally accessible.
Spin Quadrupolar orders in $d$-wave Unconventional Magnetism
Unconventional magnetism represents a class of metallic states whose Fermi surfaces exhibit spin-dependent splittings under the non-trivial representations of the rotation group. The $d$-wave $\alpha$-phase unconventional magnetic state, commonly known as altermagnet, recently, has attracted significant attention. While these systems exhibit distinct anisotropic $d$-wave characteristics in momentum space, how this microscopic topology translates into the spin distributions in real space remains a question. In this work, we bridge the intrinsic spin quadrupolar ordering in momentum space to the real-space staggered magnetic distribution. By introducing a weak, non-magnetic periodic crystal potential into a $d$-wave unconventional magnetic state, the spin-charge cross susceptibility is calculated by using the linear response theory. We reveal that the interplay between the crystal potential and the intrinsic $d$-wave spin-splitting naturally induces a spatial spin quadrupole distribution without enlarging the unit cell. Our study thus provides a physical connection between momentum-space multipoles in the even partial wave channel and real-space spin multipole orders.
Spin-charge separation in two-leg t-J ladders
Spin-charge separation is a hallmark of one-dimensional fermionic systems, yet its realization in higher dimensions remains an open question. To address this issue, we investigate a two-leg t-J ladder using the density matrix renormalization group (DMRG) method and its time-dependent extension. By analyzing ground-state correlations and single-particle removal spectra, we systematically examine the effects of plaquette diagonal hopping, spin exchange, and hole doping. Within appropriate parameter regimes, these factors drive the system from the well-known Luther Emery phase, with gapped spin and gapless charge modes, into a Luttinger liquid phase characterized by gapless spin and charge excitations, where signatures of spin-charge separation emerge. In combination with previous studies using exact diagonalization, our results provide evidence that spin-charge separation may persist in wider ladder systems.
Quantum trajectory simulation of two-dimensional non-equilibrium steady states with a trapped ion quantum processor
Digital quantum computers offer a promising route for studying complex many-body systems that are otherwise inaccessible by their classical counterparts. Capabilities including mid-circuit measurements and feedback allow for simulating the dynamics of interacting open quantum systems. Using the Quantinuum System Model H1 trapped-ion quantum computer, we experimentally realise quantum trajectories for a two-dimensional system of (interacting) particles-hard-core bosons or fermions-undergoing stochastic driving at a source and drain at opposite corners of a square lattice. We study the non-equilibrium steady state with persistent current resulting from the this in/out flow of particles. The particle statistics, presence of interactions, and introduction of a magnetic field produce measurable effects on the steady state. Our findings highlight the rich physics in this corner driven two-dimensional setup and showcases both the power and current limitations of quantum computers as a platform to study it.
Bulk-Edge Correspondence via Higher Gauge Theory
More profound than bulk topological order of quantum materials is only its unwinding via gapless excitations along boundaries of the sample. We recast this bulk-edge correspondence -- for the experimentally relevant case of fractional quantum Hall (FQH) systems -- in terms of effective relative higher gauge theory, controlled by choices of classifying fibrations. For FQH systems, we identify the complex Hopf fibration as classifying the bulk/boundary topological effects, and find that it yields a non-Lagrangian reconstruction of Floreanini-Jackiw/Wess-Zumino-Witten chiral edge currents. Remarkably, the resulting effective FQH higher gauge theory turns out to be "geometrically engineered" on M2/M5-branes probing A-type orbi-singularities in 11D supergravity, globally completed by flux-quantization in twisted equivariant differential (TED) Cohomotopy: Here the M-string ends of M2-branes on M5-branes engineer the FQH liquid's boundary. This geometric engineering on M-branes might naturally elucidate the curious combination of $W_\infty$-symmetry and of super-symmetry that is known to govern the collective excitations of FQH liquids at long wavelengths.
Thermodynamics and Tomonaga-Luttinger liquid behavior of the quantum 1D hard rod model
That author's affiliation: Centre de Physique Théorique Institution (first & last author): Centre de Physique Théorique
The one-dimensional hard rod model describes impenetrable bosons with finite diameter, extending the Lieb-Liniger model to systems with excluded volume interactions. Here, we investigate the thermodynamics of quantum HRs using Yang-Yang theory, path integral quantum Monte-Carlo calculations, and Luttinger liquid theory. We first discuss the behavior of characteristic thermodynamic quantities, exhibiting deviations to the Lieb-Liniger model for sufficiently high densities, with excellent agreement between analytical and numerical results. We then show that the hard rod model exhibits Tomonaga-Luttinger liquid behavior across a wide range of parameters, at zero and finite temperature, as unveiled by correlation functions. The Tomonaga-Luttinger parameter and thermal length can be extracted by fitting correlation functions to Tomonaga-Luttinger liquid theory, hence demonstrating a robust method for thermometry. This work provides a comprehensive study of strongly correlated hard rod systems at finite temperatures, with applications to quantum wires, spin chains, and ultracold atoms.
A Single-Molecule Spin-Photon Interface
Optical interfaces that connect long-lived spin qubits to photons are a central requirement for quantum networking and distributed quantum information processing. Currently, solid-state atomic defects are leading candidates due to their inherent spin and optical coherence. Building on these advancements, synthetically tailored molecular systems represent a fundamental change in the field, utilizing precise atomic control and consistent bottom-up assembly. However, the lack of a robust spin-photon interface combining bright fluorescence, high spectral stability, and the persistent spin lifetimes inherent to ground-state systems has prohibited the detection of individual molecular qubits. Here we show that a triplet ground state carbene molecule, embedded within a structurally matched host crystal, functions as a robust spin-photon interface with single-molecule addressability. The system exhibits narrow zero-phonon lines, spectral stability over more than an hour, spin-selective optical transitions and single-molecule optically detected magnetic resonance. Coherent control yields millisecond-scale dynamical-decoupling coherence and tens-of-milliseconds spin relaxation at a temperature of 4.5 K. These results establish molecular qubits as a viable platform for single-emitter quantum optics while preserving the advantages of bottom-up chemical design and processable materials.
Quasiparticle Quality Factors in Superconducting Resonators: Effects of Bath Temperature and Readout Power
The performance of superconducting resonators underpins a wide range of modern quantum technologies, yet their quality factor often deviates at low temperatures from standard Mattis-Bardeen predictions. This discrepancy is often attributed to nonthermal quasiparticles generated by microwave readout power, which limits the sensitivity of superconducting devices. We present a macroscopic model based on modified Rothwarf-Taylor equations that incorporates a power-dependent phonon generation term, providing an explicit relationship between quality factor, bath temperature and readout power. The model shows excellent agreement with temperature sweep measurements of NbN microstrip resonators with \b{eta}-Ta terminations over a wide dynamic range of readout power levels, accurately capturing the transition between thermally-dominated and microwave-induced loss regimes. This framework provides a predictive tool for optimizing superconducting resonators and advancing the design of high-Q devices for quantum sensing and quantum information processing.
Quantum Circuit-Based Adaptation for Credit Risk Analysis
Noisy and Intermediate-Scale Quantum, or NISQ, processors are sensitive to noise, prone to quantum decoherence, and are not yet capable of continuous quantum error correction for fault-tolerant quantum computation. Hence, quantum algorithms designed in the pre-faulttolerant era cannot neglect the noisy nature of the hardware, and investigating the relationship between quantum hardware performance and the output of quantum algorithms is essential. In this work, we experimentally study how hardware-aware variational quantum circuits on a superconducting quantum processing unit can model distributions relevant to specific use-case applications for Credit Risk Analysis, e.g., standard Gaussian distributions for latent factor loading in the Gaussian Conditional- Independence model. We use a transpilation technique tailored to the specific quantum hardware topology, which minimizes gate depth and connectivity violations, and we calibrate the gate rotations of the circuit to achieve an optimized output from quantum algorithms. Our results demonstrate the viability of quantum adaptation on a small scale, proof-of-concept model inspired by financial applications and offer a good starting point for understanding the practical use of NISQ devices.